Arylsulfonylureas and their use as herbicides and growth regulators

ABSTRACT

The invention relates to novel herbicidal and plant growth-regulating compounds of the formula (I) or salts thereof,    &lt;IMAGE&gt;  (I)  where Q, W, R, R, R, R, Y and Z are defined as in formula (I) as claimed in claim 1.

This application is a division of application Ser. No. 08/094,194, filed Sep. 21, 1993, now U.S. Pat. No. 5,463,081.

The invention relates to the field of crop protection agents, in particular selective herbicides and growth regulators of the type of the phenylsulfonylureas which are substituted by a heterocycle.

EP-A-007,687 has already disclosed, inter alia, sulfonylureas of the formula (1) ##STR2## in which R² is H, Cl, Br, F, (C₁ -C₃)alkyl, --NO₂, --SO₂ CH₃, --OCH₃, --SCH₃, --CF₃, --N(CH₃)₂, --NH₂ or --CN; R³ is H, Cl, Br, F or CH₃ ; X is CH or N, Q is O, S or optionally substituted NH; and Y and Z are H, Cl or various organic radicals. The compounds have been described as herbicides and plant growth regulators.

EP-A-0,291,851 and DE-A-3,900,472 have disclosed herbicidal and plant growth-regulating sulfonylureas of the formula (2) ##STR3## in which Z is F, Cl or Br, R¹ is H, optionally substituted alkyl, alkenyl, alkynyl or cycloalkyl, R² is H,CH₃ or C₂ H₅, R³ is H, F, Cl, Br, CH₃ or OCH₃, R⁴ is H, CH₃, (C₁ -C₄)alkoxy and X is CH or N.

U.S. Pat. No. 4,566,898 furthermore describes the sulfonylurea of the formula (3) ##STR4## as a herbicide which has outstanding properties, in particular for controlling black grass in barley and wheat.

Surprisingly, it has now been found that some iodinated arylsulfonylureas have advantageous properties.

The present invention therefore relates to compounds of the formula (I) and salts thereof, ##STR5## where Q is oxygen, sulfur or --N(R⁴)--, preferably O or S, in particular O;

W is oxygen or sulfur, preferably O;

Y and Z independently of one another are CH or N, where Y and Z are not simultaneously CH, preferably Y is CH or N and Z is N;

R is hydrogen; (C₁ -C₁₂)alkyl; (C₂ -C₁₀)alkenyl; (C₂ -C₁₀)alkynyl; (C₁ -C₆)alkyl, which is mono substituted to tetrasubstituted by radicals selected from the group comprising halogen, (C₁ -C₆)alkoxy, (C₁ -C₄)thioalkyl, --CN, (C₂ -C₅)alkoxycarbonyl and (C₂ -C₆)alkenyl; (C₃ --C₈)cycloalkyl which is unsubstituted or substituted by radicals selected from the group comprising (C₁ -C₄)alkyl, (C₁ -C₄)alkoxy, (C₁ -C₄)alkylthio and halogen; (C₅ -C₈)cycloalkenyl; phenyl (C₁ -C₄)alkyl which is unsubstituted or substituted in the phenyl radical; or a radical of the formulae A-1 to A-10 ##STR6## where X is O, S, S(O) or SO₂ ;

R¹ is hydrogen or (C₁ -C₃)alkyl;

R² is hydrogen, halogen, preferably chlorine, (C₁ -C₃)alkyl, (C₁ -C₃)alkoxy, where the two last-mentioned radicals are unsubstituted or monosubstituted or polysubstituted by halogen or (C₁ -C₃)alkoxy;

R³ is hydrogen, halogen, preferably chlorine, (C₁ -C₃)alkyl, (C₁ -C₃)alkoxy or (C₁ -C₃)alkylthio, where the abovementioned alkyl-containing radicals are unsubstituted or monosubstituted or polysubstituted by halogen or monosubstituted or disubstituted by (C₁ -C₃)alkoxy or (C₁ -C₃)alkylthio; or a radical of the formula NR⁵ R⁶, (C₃ -C₆)cycloalkyl, (C₂ -C₄)alkenyl, (C₂ -C₄)alkynyl, (C₃ -C₄)alkenyloxy or (C₃ -C₆)alkynyloxy;

R⁴ is hydrogen, (C₁ -C₄)alkyl or (C₁ -C₄)alkoxy and

R⁵ and R⁶ independently of one another are hydrogen, (C₁ -C₄)alkyl, (C₃ -C₄)alkenyl, (C₁ -C₄)haloalkyl or (C₁ -C₄)alkoxy.

In formula (I) and in what follows, alkyl, alkoxy, haloalkyl, alkylamino and alkylthio radicals as well as the corresponding unsaturated and/or substituted radicals can in each case be straight-chain or branched. Alkyl radicals, also in composite meanings such as alkoxy, haloalkyl etc., are, for example, methyl, ethyl, n- or i-propyl, n-, i-, t- or 2-butyl etc. Alkenyl and alkynyl radicals have the meanings of the unsaturated radicals which are possible and which correspond to the alkyl radicals, such as, for example, 2-propenyl, 2- or 3-butenyl, 2-propynyl and 2- or 3-butynyl. Halogen is fluorine, chlorine, bromine or iodine. Aryl is preferably a carbocyclic or heterocyclic aromatic ring which can optionally be fused with an aliphatic or aromatic ring; in particular, aryl is phenyl. Substituted phenyl is phenyl which is substituted for example by one or more, preferably one to three, radicals selected from the group comprising halogen, (C₁ -C₄)alkyl, (C₁ -C₄)alkoxy, (C₁ -C₄)haloalkyl, (C₁ -C₄)thioalkyl, (C₂ -C₅)alkoxycarbonyl, (C₂ -C₅)alkylcarbonyloxy, carboxamide, (C₂ -C₅)alkylcarbonylamino, (C₂ -C₅)alkylaminocarbonyl, di- (C₁ -C₄)alkyl!aminocarbonyl and nitro. The same applies analogously to substituted aryl.

The compounds of the formula (I) can form salts in which the hydrogen of the --SO₂ --NH-- group is replaced by a cation which is suitable for agriculture. Examples of these salts are metal salts, in particular alkali metal salts or alkaline earth metal salts, but also ammonium salts or salts with organic amines. Salt formation can also be effected by an addition reaction of a strong acid with the heterocycle moiety of the compounds of the formula (I). Examples of acids which are suitable for this purpose are HCl, HNO₃, trichloroacetic acid, acetic acid or palmitic acid.

Some compounds of the formula (I) can contain one or more asymmetric carbon atoms or else double bonds which are not mentioned individually in the formula (I). However, formula (I) embraces all possible stereoisomers which are defined by their specific spatial form such as enantiomers, diastereomers, Z and E isomers, which can be obtained from mixtures of the stereoisomers by customary methods or, alternatively, by stereoselective reactions in combination with the use of stereochemically pure starting materials. The invention thus relates to the stereo-isomers mentioned in pure form and also their mixtures.

Compounds of the formula (I) according to the invention, or salts thereof, which are of particular interest are those where

R is hydrogen; (C₁ -C₆)alkyl; (C₂ -C₆)alkenyl; (C₂ -C₆)alkynyl; (C₁ -C₄)alkyl which is monosubstituted to tetrasubstituted, preferably monosubstituted, by radicals selected from the group comprising halogen, (C₁ -C₂)alkoxy, (C₁ -C₂)thioalkyl, (C₂ -C₃)alkoxycarbonyl and (C₂ -C₄)alkenyl; (C₅ -C₆)cycloalkyl which is unsubstituted or substituted by radicals selected from the group comprising (C₁ -C₄)alkyl, (C₁ -C₄)alkoxy, (C₁ -C₄)alkylthio and halogen; (C₅ -C₆)cycloalkenyl; benzyl which is unsubstituted or substituted in the phenyl radical by one to three radicals selected from the group comprising halogen, (C₁ -C₂)alkyl, (C₁ -C₂)alkoxy, (C₁ -C₂)haloalkyl, (C₁ -C₂)thioalkyl and (C₂ -C₄)alkoxycarbonyl, or a radical of the abovementioned formulae A-1 to A-10, where

X is O, S, S(O) or SO₂, preferably O.

Compounds of the formula (I) according to the invention, or salts thereof, which are of particular interest are those where

R¹ is hydrogen or CH₃ ;

R² is hydrogen, halogen, preferably chlorine, (C₁ -C₂)alkyl, (C₁ -C₂)alkoxy, where the two last-mentioned radicals are unsubstituted or monosubstituted or polysubstituted by halogen or (C₁ -C₃)alkoxy;

R³ is hydrogen, halogen, preferably chlorine, (C₁ -C₂)alkyl, (C₁ -C₂)alkoxy or (C₁ -C₂)alkylthio, where the abovementioned alkyl-containing radicals are unsubstituted or monosubstituted or polysubstituted by halogen or monosubstituted or disubstituted by (C₁ -C₂)alkoxy or (C₁ -C₂)alkylthio; or a radical of the formula NR⁵ R⁶ ;

R⁴ is hydrogen or (C₁ -C₂)alkyl and

R⁵ and R⁶ independently of one another are hydrogen or (C₁ -C₂)alkyl.

Preferred compounds of the formula (I) according to the invention or salts thereof are those in which

W is oxygen and

R¹ is hydrogen or CH₃.

Particularly preferred compounds of the formula (I) or salts thereof are those in which

Y is CH or N,

Z is N and

R² is hydrogen, CH₃, CH₂ CH₃, OCH₃, OCH₂ CH₃, OCHF₂, Cl and

R³ is hydrogen, CH₃, CH₂ CH₃, OCH₃, OCH₂ CH₃, OCHF₂, NH(CH₃), N(CH₃)₂, CF₃, OCH₂ CF₃ or Cl.

Other preferred compounds according to the invention are those which exhibit a combination of the abovementioned preferred features.

The present invention furthermore relates to processes for the preparation of the compounds of the formula (I) or salts thereof, which comprise

a) reacting a compound of the formula (II) ##STR7## with a heterocyclic carbamate of the formula (III) ##STR8## where R' is unsubstituted or substituted aryl or alkyl, preferably unsubstituted or substituted phenyl or (C₁ -C₄)alkyl, in particular phenyl or methyl, or

b) reacting a phenylsulfonyl carbamate of the formula (IV) ##STR9## with an aminoheterocycle of the formula (V) ##STR10## or c) reacting a sulfonyl isocyanate of the formula (VI) ##STR11## with an aminoheterocycle of the formula (V) mentioned under b).

The compounds of the formula (II) and (III) are reacted by means of base catalysis in an inert solvent, such as, for example, acetonitrile, dioxane or tetrahydrofuran at temperatures of between 0° C. and the boiling point of the solvent. 1,8-Diazabicyclo 5.4.0!undec-7-ene (DBU) is preferably used as the base.

The sulfonamides (II) are novel compounds; this invention also relates to these compounds and to their preparation (see Tables 1a and 1b further below). They are obtained starting from corresponding sulfonyl halides, preferably corresponding sulfochlorides, which react either directly with ammonia or with tert.-butylamine, followed by elimination of the protective groups, for example by treatment with trifluoroacetic acid, to give the sulfonamides of the formula (II). The sulfonyl halides which can be used in the process can be obtained from the corresponding anilines by diazotization and exchange of the diazo group with sulfur dioxide in the presence of a catalyst such as copper(I) chloride in hydrochloric acid or acetic acid, cf. Meerwein, Chem. Ber. 90, 841-52 (1957).

The carbamates of the formula (III) can be prepared by methods as are described in the South African Patent Applications 82/5671 and 82/5045 (or EP-A-0,072,347 and EP-A-0,070,802, respectively).

The compounds (IV) are preferably reacted with the amino-heterocycles (V) in inert, aprotic solvents, such as, for example, dioxane, acetonitrile or tetrahydrofuran, at temperatures of between 0° C. and the boiling point of the solvent. The starting compounds required, of the formula (V), are known or can be prepared by methods known in principle, see "The Chemistry of Heterocyclic Compounds", Vol. XVI, (1962), Interscience Publ., New York & London, and Supplement I of this manual. Amino-substituted triazine derivatives are reviewed by Smolin and Rapaport in "The Chemistry of Heterocyclic Compounds", Vol. XIII, (1959), Interscience Publ., New York & London. The iodinated phenylsulfonyl carbamates (IV) are obtained analogously to processes given in EP-A-0,044,808 or EP-A-0,237,292.

The iodinated arylsulfonyl isocyanates of the formula (VI) are novel compounds and also a subject of the invention. They can be prepared analogously to methods of EP-A-0,184,385 and reacted with the abovementioned amino-heterocycles of the formula (V).

The salts of the compounds of the formula (I) are preferably prepared in inert solvents, such as, for example, water, methanol, dichloromethane or acetone, at temperatures of 0°-100°. Examples of suitable bases for the preparation of the salts according to the invention are alkali metal carbonates, such as potassium carbonate, alkali metal hydroxides and alkaline earth metal hydroxides, ammonia or ethanolamine. Acids which are particularly suitable for salt formation are HCl, HNO₃, trichloroacetic acid, acetic acid or palmitic acid.

The compounds of the formula (I) according to the invention have an excellent herbicidal activity against a broad range of economically important monocotyledon and dicotyledon weeds. The active substances act equally well on perennial weeds which produce shoots from rhizomes, rootstocks or other perennial organs and which cannot be easily controlled. In this context, it does not matter if the substances are applied before sowing, as a pre-emergence treatment or post-emergence treatment. Some representatives of the monocotyledon and dicotyledon weed flora which can be controlled by the compounds according to the invention may be mentioned individually as examples, but this is not to be taken to mean a restriction to certain species.

The monocotyledon weed species controlled include, for example, Avena, Lolium, Alopecurus, Phalaris, Echinochloa, Digitaria, Setaria etc. and Cyperus species from the annual group, and the perennial species include Agropyron, Cynodon, Imperata and Sorghum etc., and also perennial Cyperus species.

Of the dicotyledon weed species, the range of action covers, for example, Galium, Viola, Veronica, Lamium, Stellaria, Amaranthus, Sinapis, Ipomoea, Matricaria, Abutilon, Sida etc. from the annual plants and Convolvulus, Cirsium, Rumex, Artemisia etc. from the perennial weeds.

Excellent control of weeds occurring under the specific culture conditions in rice, such as, for example, Sagittaria, Alisma, Eleocharis, Scirpus, Cyperus etc., by the active substances according to the invention is also possible.

If the compounds according to the invention are applied to the soil surface before germination, either emergence of the weed seedlings is prevented completely, or the weeds grow until they have reached the cotyledon stage but growth then comes to a standstill and, after a period of three to four weeks, the plants eventually die completely. When, in the post-emergence method, the active substances are applied to the green parts of the plants, growth also stops dramatically very soon after the treatment, and the weed plants remain in the growth stage of the time of application, or, after a certain period of time, die more or less rapidly so that competition by the weeds, which is detrimental for the crop plants, can thus be prevented at a very early stage and in a sustained manner by using the novel compounds according to the invention.

Even though the compounds according to the invention have an excellent herbicidal activity against monocotyledon and dicotyledon weeds, crop plants of economically important crops such as, for example, wheat, barley, rye, maize, rice, sugar beet, cotton and soya, are damaged to a negligible extent only, or not at all. Thus, the present compounds are very suitable for selectively controlling undesired plant growth in agricultural plantations of useful plants.

In addition, the compounds according to the invention have plant growth-regulating properties in crop plants. They intervene in the plant metabolism in a regulating manner and can thus be employed for facilitating harvesting, such as, for example, by provoking desiccation, abscission and stunted growth. Furthermore, they are suitable for generally regulating and inhibiting undesired vegetative growth, without simultaneously destroying the plants. Inhibition of vegetative growth plays an important role in many monocotyledon and dicotyledon crops because lodging can be reduced hereby, or prevented completely.

The compounds according to the invention can be formulated in many ways, depending on the prevailing biological and/or chemicophysical parameters. Examples of possible formulations are the following: wettable powders (WP), water-soluble powders (SP), water-soluble concentrates, emulsifiable concentrates (EC), emulsions (EW) such as oil-in-water and water-in-oil emulsions, sprayable solutions or emulsions, suspension concentrates (SC), dispersions on an oil or water basis, oil-miscible solutions, suspoemulsions, capsule suspensions (CS), dusts (DP), seed-dressing agents, granules for broadcasting and soil application, granules (GR) in the form of microgranules, spray granules, coated granules and adsorption granules, water-dispersible granules (WG), water-soluble granules (SG), ULV formulations, microcapsules and waxes.

These individual types of formulation are known in principle and are described, for example, in: Winnacker-Kuchler, "Chemische Technologie", Chemical Technology!, Volume 7, G. Hauser Verlag Munich, 4th Ed. 1986; van Valkenburg, "Pesticides Formulations", Marcel Dekker N.Y., 2nd Ed. 1972-73; K. Martens, "Spray Drying Handbook", 3rd Ed. 1979, G. Goodwin Ltd. London.

The formulation auxiliaries required, such as inert materials, surfactants, solvents and further additives, are also known and are described, for example, in: Watkins, "Handbook of Insecticide Dust Diluents and Carriers", 2nd Ed., Darland Books, Galdwell N. J.; H. v. Olphen, "Introduction to Clay Colloid Chemistry"; 2nd Ed., J. Wiley & Sons, N.Y.; Marsden, "Solvents Guide", 2nd Ed., Interscience, N.Y. 1950; McCutcheon's "Detergents and Emulsifiers Annual", MG Publ. Corp., Ridgewood N.J.; Sisley and Wood, "Encyclopedia of Surface Active Agents", Chem. Publ. Co. Inc., N.Y. 1964; Schonfeldt, "Grenzflachenaktive Athylenoxidaddukte", Surface-active Ethylene Oxide Adducts!, Wiss. Verlagsgesell., Stuttgart 1976; Winnacker-Kuchler, "Chemische Technologie", Chemical Technology!, Volume 7, G. Hauser Verlag Munich, 4th Ed. 1986.

Wettable powders are preparations which are uniformly dispersible in water and which, besides the active substance, also contain wetting agents, for example, polyoxyethylated alkylphenols, polyoxyethylated fatty alcohols and fatty a mines, fatty alcohol polyglycol ether sulfates, alkanesulfonates or alkylarylsulfonates, and dispersing agents, for example sodium ligninsulfonate, sodium 2,2'-dinaphthylmethane-6,6'-disulfonate, sodium dibutylnaphthalenesulfonate and also sodium oleylmethyltauride, in addition to a diluent or inert substance.

Emulsifiable concentrates are prepared, for example, by dissolving the active substance in an organic solvent, for example butanol, cyclohexanone, dimethylformamide, xylene and also higher-boiling aromatics or hydrocarbons, with the addition of one or more emulsifiers. Emulsifiers which can be used are, for example: calcium salts of alkylarylsulfonic acids, such as calcium dodecylbenzenesulfonate or non-ionic emulsifiers, such as fatty acid polyglycol esters, alkylaryl polyglycol ethers, fatty alcohol polyglycol ethers, propylene oxide/ethylene oxide condensation products (for example block polymers), alkyl polyglycol ethers, sorbitan fatty acid esters, polyoxyethylene sorbitan fatty acid esters or polyoxyethylene sorbitol esters.

Dusts are obtained by grinding the active substance with finely divided solid substances, for example talc or natural clays, such as kaolin, bentonite or pyrophyllite, or diatomaceous earth.

Granules can be produced either by spraying the active substance onto adsorptive, granulated inert material or by applying active substance concentrates onto the surface of carriers such as sand, kaolinites or of granulated inert material, by means of binders, for example polyvinyl alcohol, sodium polyacrylate or alternatively mineral oils. Suitable active substances can also be granulated in the manner which is conventional for the production of fertilizer granules, if desired in a mixture with fertilizers.

Disk granules, fluidized-bed granules, extruder granules and spray granules can be prepared by conventional methods; see, for example, methods in "Spray Drying Handbook", 3rd Ed. 1979, G. Goodwin Ltd., London; J. E. Browning, "Agglomeration", Chemical and Engineering 1967, pages 147 et seq.; "Perry's Chemical Engineer's Handbook", 5th Ed., McGraw-Hill, New York 1973, p. 8-57.

Further information on the formulation of crop protection agents can be found, for example, in G. G. Klingman, "Weed Control as a Science", John Wiley and Sons, Inc., New York, 1961, pages 81-96 and J. D. Freyer's, A. Evans, "Weed Control Handbook", 5th Ed., Blackwell Scientific Publications, Oxford, 1968, pages 101-103.

The active substance concentration in wettable powders is, for example, about 10 to 90% by weight; the remainder to 100% by weight is composed of conventional formulation components. In the case of emulsifiable concentrates, the active substance concentration can be about 1 to 80% by weight. Formulations in the form of dusts usually contain 1 to 20% by weight of active substance, sprayable solutions about 0.2 to 20% by weight. In the case of granules the active substance content depends partly on whether the active compound is liquid or solid. The water-dispersible granules usually contain between 10 and 90% by weight of active substance.

In addition, the active substance formulations mentioned contain, if appropriate, the adhesives, wetting agents, dispersing agents, emulsifiers, penetrants, solvents, fillers or carriers which are conventional in each case.

Based on these formulations, it is also possible to prepare combinations with other substances which are active in arable farming, for example pesticides such as insecticides, acaracides, fungicides and herbicides, and/or fertilizers and/or growth regulators, for example in the form of a readymix or as a tank mix.

In particular, the compounds of the formula (I) according to the invention can be used together with further herbicides as are known, for example, from Weed Research 26, 441-5 (1986) or "The Pesticide Manual", 9th Edition, The British Crop Protection Council, 1990, England. The following active substances may be mentioned as examples of herbicides which are known from the literature and which can be combined according to the invention with the compounds of the formula (I) (the common name, or manufacturer's code, of each of the active substances is in bold print and the chemical name is then in ordinary typeface, see scheme):

Common name (or Manufacturer's code) Chemical name Scheme!

AC 263222 2- 4,5-dihydro-4-methyl-4-(1-methylethyl)-5-oxo-1H-imidazol-2-yl!-5-methyl-3-pyridinecarboxylic acid;

acetochlor 2-chloro-N-(ethoxymethyl)-N-(2-ethyl-6-methylphenyl)acetamide;

acifluorfen 5- 2-chloro-4-(trifluoromethyl)phenoxy!-2-nitrobenzoic acid;

aclonifen 2-chloro-6-nitro-3-phenoxyaniline;

AKH 7088 methyl 1- 5- 2-chloro-4-(trifluoromethyl)phenoxy!-2-nitrophenyl!-2-methoxyethylidene!amino!oxy!acetate;

alachlor 2-chloro-N-(2,6-diethylphenyl)-N-(methoxymethyl)acetamide;

alloxydim methyl 3- 1-(allyloxyimino)-butyl!-4-hydroxy-6,6-dimethyl-2-cyclohex-3-enecarboxylate;

ametryn N-ethyl-N'-(1-methylethyl)-6-(methylthio)-1,3,5-triazine-2,4-diamine;

amidosulfuron 1- N-Methyl-N-(methylsulfonyl)-aminosulfonyl!-3-(4,6-dimethoxypyrimidin-2-yl)urea;

amitrole 1H-1,2,4-triazol-3-amine;

AMS ammonium sulfamate;

anilofos S- 2- (4-chlorophenyl)(1-methylethyl)amino!-2-oxoethyl!O,O-dimethylphosphorodithioate;

asulam methyl (4-aminophenyl)sulfonyl!carbamate;

atrazine 6-chloro-N-ethyl-N'-(1-methylethyl)-1,3,5-triazine-2,4-diamine;

aziprotryn 2-azido-N-(1-methylethyl)-6-methylthio-1,3,5-triazin-2-amine;

barban 4-chloro-2-butynyl 3-chlorophenylcarbamate;

BAS 516 H 5-fluoro-2-phenyl-4H-3,1-benzoxazin-4-one;

benazolin 4-chloro-2-oxo-3(2H)-benzothiazoleacetic acid;

benfluralin N-butyl-N-ethyl-2,6-dinitro-4-(trifluoromethyl)benzenamine;

benfuresate 2,3-dihydro-3,3-dimethylbenzofuran-5-yl ethanesulfonate;

bensulfuron-methyl methyl 2- (4,6-dimethoxy-2-pyrimidinyl)amino!carbonyl!amino!sulfonyl!methyl!benzoate;

bensulide O,O-bis-(1-methylethyl)S- 2- (phenylsulfonyl)amino!ethyl!phosphorodithioate;

bentazone 3-(1-methylethyl)-1H-2,1,3-benzothiadiazin-4(3H)-one, 2,2-dioxide;

benzofenap 2- 4-(2,4-dichloro-3-methylbenzoyl)-1,3-dimethyl-1H-pyrazol-5-yl!oxy!-1-(4-methylphenyl)ethanone;

benzofluor N- 4-(ethylthio)-2-(trifluoromethyl)phenyl!methanesulfonamide;

benzoylprop-ethyl ethyl N-benzoyl-N-(3,4-dichlorophenyl)alaninate;

benzthiazuron N-2-benzothiazolyl-N'-methylurea;

bialaphos 4-(hydroxymethylphosphinyl)-L-2-aminobutanoyl-L-alanyl-L-alanine;

bifenox methyl 5-(2,4-dichlorophenoxy)-2-nitrobenzoate;

bromacil bromo-6-methyl-3-(1-methylpropyl)-2,4(1H,3H)-pyrimidinedione;

bromobutide N- (1,1-dimethyl)methylphenyl!-2-bromo-3,3-dimethylbutyramide;

bromofenoxim 3,5-dibromo-4-hydroxybenzaldehyde O-(2,4-dinitrophenyl)oxime;

bromoxynil 3,5-dibromo-4-hydroxybenzonitrile;

bromuron N'-(4-bromophenyl)-N,N-dimethylurea;

buminafos dibutyl 1-(butylamino)cyclohexyl!phosphonate;

butachlor N-(butoxymethyl)-2-chloro-N-(2,6-diethylphenyl)acetamide;

butamifos O-ethyl O-(5-methyl-2-nitrophenyl) (1-methylpropyl)phosphoramidothioate;

butenachlor (Z)-N-but-2-enyloxymethyl-2-chloro-2',6'-diethylacetanilide;

busoxinone 3- 5-(1,1-dimethylethyl)-isoxazol-3-yl!-4-hyroxy-1-methyl-2-imidazolidinone;

buthidazole 3- 5-(1,1-dimethylethyl)-1,3,4-thiadiazol-2-yl!-4-hydroxy-1-methyl-2-imidazolidinone;

butralin 4-(1,1-dimethylethyl)-N-(1-methylpropyl)-2,6-dinitrobenzenamine;

butylate S-ethyl bis(2-methylpropyl)carbamothioate;

C 4874 (tetrahydro-2-furanyl)methyl 2- 4- (6-chloro-2-quinoxalinyl)oxy!phenoxy!propanoate;

carbetamide (R)-N-ethyl-2- (phenylamino)carbonyl!oxy!propanamide;

CDAA 2-chloro-N,N-di-2-propenylacetamide;

CDEC 2-chloroallyl diethyldithiocarbamate;

CGA 184927 2-propynyl 2- 4- (5-chloro-3-fluoro-2-pyridinyl)oxy!phenoxy!propanoate;

chlomethoxyfen 4-(2,4-dichlorophenoxy)-2-methoxy-1-nitrobenzene;

chloramben 3-amino-2,5-dichlorobenzoic acid;

chlorbromuron 3-(4-bromo-3-chlorophenyl)-1-methoxy-1-methylurea;

chlorbufam 1-methyl-2-propynyl (3-chlorophenyl)carbamate;

chlorfenac 2,3,6-trichlorobenzeneacetic acid;

chlorflurecol-methyl methyl 2-chloro-9-hydroxy-9H-fluorene-9-carboxylate;

chloridazon 5-amino-4-chloro-2-phenyl-3(2H)-pyridazinone;

chlorimuron ethyl ethyl 2- (4-chloro-6-methoxy-2-pyrimidinyl)amino!carbonyl!amino!sulfonyl!benzoate;

chlornitrofen 1,3,5-trichloro-2-(4-nitrophenoxy)benzene;

chlorotoluron N'-(3-chloro-4-methylphenyl)-N,N-dimethylurea;

chloroxuron N'- 4-(4-chlorophenoxy)phenyl!-N,N-dimethylurea;

chlorpropham 1-methylethyl 3-chlorophenylcarbamate;

chlorsulfuron 2-chloro-N- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)amino!carbonyl!benzenesulfonamide;

chlorthal-dimethyl dimethyl 2,3,5,6-tetrachloro-1,4-benzenedicarboxylate;

chlorthiamid 2,6-dichlorobenzenecarbothioamide;

cinmethylin exo-1-methyl-4-(1-methylethyl)-2- (2-methylphenyl)methoxy!-7-oxabicyclo 2.2.1!heptane;

cinosulfuron 1-(4,6-dimethoxy-1,3,5-triazin-2-yl)3- 2-(2-methoxyethoxy)phenylsulfonyl!urea;

clethodim (E,E)-2- 1- (3-chloro-2-propenyl)oxy!imino!propyl!-5- 2-(ethylthio)propyl!-3-hydroxy-2-cyclohexen-1-one;

clomazone 2- (2-chlorophenyl)methyl!-4,4-dimethyl-3-isoxazolidinone;

clomeprop (2,4-dichloro-3-methylphenyl)oxy!-2-propionanilide;

cloproxydim (E,E)-2- 1- (3-chloro-2-propenyl)oxy!imino!butyl!-5- 2-(ethylthio)propyl!-3-hydroxy-2-cyclohexen-1-one;

clopyralid 3,6-dichloro-2-pyridinecarboxylic acid;

cyanazine 2- 4-chloro-6-(ethylamino)-1,3,5-triazin-2-yl!amino!-2-methylpropanenitrile;

cycloate S-ethyl cyclohexylethylcarbamothioate;

cycloxydim 2- 1-(ethoxyimino)butyl!-5-(tetrahydrothiopyran-3-yl)-3-hydroxy-2-cyclohexen-1-one;

cycluron 3-cyclooctyl-1-dimethylurea;

cyperquat 1-methyl-4-phenylpyridinium;

cyprazine 2-chloro-4-(cyclopropylamino)-6-(isopropylamino)-s-triazine;

cyprazole N- 5-(2-chloro-1,1-dimethylethyl)-1,3,4-thiadiazol-2-yl!-cyclopropanecarboxamide;

2,4-DB 4-(2,4-dichlorophenoxy)butanoic acid;

dalapon 2,2-dichloropropanoic acid;

desmediphamethyl 3- (phenylamino)carbonyl!oxy!phenyl!carbamate;

desmetryn 2-(isopropylamino)-4-(methylamino)-6-(methylthio)s-triazine;

di-allate S-(2,3-dichloro-2-propenyl)bis(1-methylethyl)carbamothioate;

dicamba 3,6-dichloro-2-methoxybenzoic acid;

dichlobenil 2,6-dichlorobenzonitrile;

dichlorprop 2-(2,4-dichlorophenoxy)propanoic acid;

diclofop-methyl methyl 2- 4-(2,4-dichlorophenoxy)phenoxy!-propanoate;

diethatyl N-(chloroacetyl)-N-(2,6-diethylphenyl)glycine;

difenoxuron N'- 4-(4-methoxyphenoxy)phenyl!-N,N-dimethylurea;

difenzoquat 1,2-dimethyl-3,5-diphenyl-1H-pyrazolium;

diflufenican N-(2,4-difluorophenyl)-2- 3-(trifluoromethyl)-phenoxy!-3-pyridinecarboxamide;

dimefuron N'- 3-chloro-4- 5-(1,1-dimethylethyl)-2-oxo-1,3,4-oxadiazol-3(2H)-yl!phenyl!-N,N-dimethylurea;

dimethachlor 2-chloro-N-(2,6-dimethylphenyl)-N-(2-methoxyethyl)acetamide;

dimethametryn N-(1,2-dimethylpropyl)-N'-ethyl-6-(methylthio)-1,3,5-triazine-2,4-diamine;

dimethipin 2,3-dihydro-5,6-dimethyl-1,4-dithiin, 1,1,4,4-tetraoxide;

dinitramine N³,N³ -diethyl-2,4-dinitro-6-(trifluoromethyl)-1,3-benzenediamine;

dinoseb 2-(1-methylpropyl)-4,6-dinitrophenol;

dinoterb 2-(1,1-dimethylethyl)-4,6-dinitrophenol;

diphenamid N,N-dimethyl-2,2-diphenylacetamide;

dipropetryn 6-ethylthio-N,N'-bis(1-methylethyl)-1,3,5-triazine-2,4-diamine;

diquat 6,7 dihydrodipyrido 1,2-a:2',1'-c!pyrazinediium,

dithiopyr 2-(difluoromethyl)-4-(2-methylpropyl)-6-(trifluoromethyl)-3,5-pyridinedicarbothioic acid;

diuron N'-(3,4-dichlorophenyl)-N,N-dimethylurea;

DNOC 2-methyl-4,6-dinitrophenol;

DPX-A7881methyl 2- (4-ethoxy-6-N-(methyl)amino-1,3,5-triazin-2-yl!amino!carbonyl!amino!sulfonyl!benzoate;

DPX-E9636 N- (4,6-dimethoxy-2-pyrimidinyl)amino!carbonyl!-3-(ethylsulfonyl)-2-pyridinesulfonamide;

dymron N-(4-methylphenyl)-N'-(1-methyl-1-phenylethyl)urea;

eglinazine-ethyl ethyl N- 4-chloro-6-(ethylamino)-1,3,5-tria-zin-2-yl!glycinate;

EL 177 5-cyano-1-(1,1-dimethylethyl)-N-methyl-3H-pyrazole-4-carbo xamide;

endothal 7-oxabicyclo 2.2.1!heptane-2,3-dicarboxylic acid;

EPTC S-ethyl dipropylcarbamothioate;

esprocarb S-(methylphenyl)N-ethyl-N-(1,2-dimethyl)propylcarbamothioate;

ethalfluralin N-ethyl-N-(2-methyl-2-propenyl)-2,6-dinitro-4-(trifluoromethyl)benzenamine;

ethidimuron N- 5-(ethylsulfonyl)-1,3,4-thiadiazol-2-yl!-N,N'-dimethylurea;

ethiozin 4-amino-6-(1,1-dimethylethyl)-3-(ethylthio)-1,2,4-triazin-5(4H)-one;

ethofumesate 2-ethoxy-2,3-dihydro-3,3-dimethyl-5-benzofuranyl methanesulfonate;

F 5231 N- 2-chloro-4-fluoro-5- 4-(3-fluoropropyl)-4,5-dihydro-5-oxo-1H-tetrazol-1-yl!phenyl-!ethanesulfonamide;

fenoprop 2-(2,4,5-trichlorophenoxy)propanoic acid;

fenoxaprop-ethyl ethyl 2- 4- (6-chloro-2-benzoxazolyl)oxy!-phenoxy!propanoate;

fenuron N,N-dimethyl-N'-phenylurea;

flamprop-methyl methyl N-benzoyl-N-(3-chloro-4-fluorophenyl)-alaninate;

flazasulfuron 1-(4,6-dimethoxypyrimidin-2-yl)-3- 3-(trifluoromethyl)-2-pyridylsulfonyl!urea;

fluazifop-butyl butyl 2- 4- 5-(trifluoromethyl)-2-pyridinyl!-oxy!phenoxy!propanoate;

fluchloralin N-(2-chloroethyl)-2,6-dinitro-N-propyl-4-(trifluoromethyl)benzenamine;

flumeturon N,N-dimethyl-N'- 3-(trifluoromethyl)phenyl!urea;

flumipropyn 2- 4-chloro-2-fluoro-5- (1-methyl-2-propynyl)oxy!phenyl-4,5,6,7-tetrahydro-1H-isoindole-1,3(2H)-dione;

fluorodifen 2-nitro-1-(4-nitrophenoxy)-4-(trifluoromethyl)benzene;

fluoroglycofen-ethyl ethyl carboxymethyl 5- 2-chloro-4-(trifluoromethyl)phenoxy!-2-nitrobenzoate;

fluridone 1-methyl-3-phenyl-5- 3-(trifluoromethyl)-phenyl!-4(1H)-pyridinone;

flurochloridone 3-chloro-4-(chloromethyl)-1- 3-(trifluoromethyl)phenyl!-2-pyrrolidinone;

fluroxypyr 4-amino-3,5-dichloro-6-fluoro-2-pyridyloxyacetic acid;

flurtamone 5-(methylamino)-2-phenyl-4- 3-(trifluoromethyl)phenyl!-3(2H)-furanone;

fomesafen 5- 2-chloro-4-(trifluoromethyl)phenoxy!-N-(methylsulfonyl)-2-nitrobenzamide;

fosamine ethyl hydrogen carbamoylphosphonate;

furyloxyfen 3- 5- 2-chloro-4-(trifluoromethyl)phenoxy!-2-nitrophenoxy!-tetrahydrofuran;

glufosinate 4- hydroxy(methyl)phosphinoyl!homoalanine;

glyphosate N-(phosphonomethyl)glycine;

halosaten 5- 6-chloro-2-fluoro-4-(trifluoromethyl)phenoxy!-N-(ethylsulfonyl)-2-nitrobenzamide;

haloxyfop 2- 4- 3-chloro-5-(trifluoromethyl)-2-pyridinyl!oxy!phenoxy!propanoic acid;

hexazinone 3-cyclohexyl-6-(dimethylamino)-1-methyl-1,3,5-triazine-2,4(1H,3H)-dione;

Hw 52 N-(2,3-dichlorophenyl)-4-(ethoxymethoxy)benzamide;

imazamethabenz-methyl methyl 6-(4-isopropyl-4-methyl-5-oxo-2-imidazolin-2-yl)-m-toluate and methyl 6-(4-isopropyl-4-methyl-5-oxo-2-imidazolin-2-yl)-p-toluate;

imazapyr 2- 4,5-dihydro-4-methyl-4-(1-methylethyl)-5-oxo-1H-imidazol-2-yl!-3-pyridinecarboxylic acid;

imazaquin 2- 4,5-dihydro-4-methyl-4-(1-methylethyl)-5-oxo-1H-imidazol-2-yl!-3-quinolinecarboxylic acid;

imazethapyr 2- 4,5-dihydro-4-methyl-4-(1-methylethyl)-5-oxo-1H-imidazol-2-yl!-5-ethyl-3-pyridinecarboxylic acid;

imazosulfuron 2-chloro-N- (4,6-dimethoxy-2-pyrimidinyl)amino!carbonyl!imidazo 1,2-a!pyridine-3-sulfonamide;

ioxynil 4-hydroxy-3,5-diiodobenzonitrile;

isocarbamid N-(2-methylpropyl)-2-oxo-1-imidazolidinecarboxamide;

isopropalin 4-(1-methylethyl)-2,6-dinitro-N,N-dipropylbenzenamine;

isoproturon N- 4-(methylethyl)phenyl!-N',N'-dimethylurea;

isouron N'- 5-(1,1-dimethylethyl)-3-isoxazolyl!-N,N-dimethylurea;

isoxaben N- 3-(1-ethyl-1-methylpropyl)-5-isoxazolyl!-2,6-dimethoxybenzamide;

isoxapyrifop 2- 2- 4- (3,5-dichloro-2-pyridinyl)oxy!phenoxy!-1-oxopropyl!-isoxazolidine;

karbutilate 3- (dimethylamino)carbonyl!amino!phenyl (1,1-dimethylethyl)carbamate;

lactofen 2-ethoxy-1-methyl-2-oxoethyl 5- 2-chloro-4-(trifluoromethyl)phenoxy!-2-nitrobenzoate;

lenacil 3-cyclohexyl-6,7-dihydro-1H-cyclopentapyrimidine-2,4(3H,5H)-dione;

linuron N'-(3,4-dichlorophenyl)-N-methoxy-N-methylurea;

MCPA (4-chloro-2-methylphenoxy)acetic acid;

MCPB 4-(4-chloro-2-methylphenoxy)butanoic acid;

mecoprop 2-(4-chloro-4-methylphenoxy)propanoic acid;

mefenacet 2-benzothiazol-2-yloxy-N-methylacetanilide;

mefluidide N- 2,4-dimethyl-5- trifluoromethyl)sulfonyl!amino!phenyl!acetamide;

metamitron 4-amino-3-methyl-6-phenyl-1,2,4-triazin-5(4H)-one;

metazachlor 2-chloro-N-(2,6-dimethylphenyl)-N-(1(H)-pyrazol-1-ylmethyl)acetamide;

methabenzthiazuron 1,3-dimethyl-3-(2-benzothiazolyl)urea;

metham methylcarbamodithioic acid;

methazole 2-(3,4-dichlorophenyl)-4-methyl-1,2,4-oxadiazolidine-3,5-dione;

methoxyphenone (4-methoxy-3-methylphenyl)(3-methylphenyl)methanone;

methyldymron N-methyl-N'-(1-methyl-1-phenylethyl)-N-phenylurea;

metobromuron N'-(4-bromophenyl)-N-methoxy-N-methylurea;

metolachlor 2-chloro-N-(2-ethyl-6-methylphenyl)-N-(2-methoxy-1-methylethyl)acetamide;

metoxuron N'-(3-chloro-4-methoxyphenyl)-N,N-dimethylurea;

metribuzin 4-amino-6-(1,1-dimethylethyl)-3-(methylthio)-1,2,4-triazin-5(4H)-one;

metsulfuron-methyl methyl 2- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)amino!carbonyl!amino!sulfonyl!benzoate;

MH 1,2-dihydro-3,6-pyridazinedione;

molinate S-ethyl hexahydro-1H-azepine-1-carbothioate;

monalide N-(4-chlorophenyl)-2,2-dimethylpentanamide;

monolinuron 3-(4-chlorophenyl)-1-methoxy-1-methylurea;

monuron N'-(4-chlorophenyl)-N,N-dimethylurea;

MT 128 6-chloro-N-(3-chloro-2-propenyl)-5-methyl-N-phenyl-3-pyridazinamine;

MT 5950 N- 3-chloro-4-(1-methylethyl)phenyl!-2-methylpentanamide;

naproanilide 2-(2-naphthalenyloxy)-N-phenylpropanamide;

napropamide N,N-diethyl-2-(1-naphthalenyloxy)propanamide;

naptalam 2- (1-naphthalenylamino)carbonyl!benzoic acid;

NC 310 4-(2,4-dichlorobenzoyl)-1-methyl-5-benzyloxypyrazole;

neburon 1-butyl-3-(3,4-dichlorophenyl)-1-methylurea;

nicosulfuron 2- (4,6-dimethoxy-2-pyrimidinyl)amino!carbonyl!amino!sulfonyl!-N,N-dimethyl-3-pyridinecarboxamide;

nipyraclophen 5-amino-1-(2,6-dichloro-4-(trifluoromethyl)phenyl)-4-nitropyrazole;

nitralin 4-(methylsulfonyl)-2,6-dinitro-N,N-dipropylaniline;

nitrofen 2,4-dichloro-1-(4-nitrophenoxy)benzene;

nitrofluorfen 2-chloro-1-(4-nitrophenoxy)-4-(trifluoromethyl)benzene;

norflurazon 4-chloro-5-(methylamino)-2- 3-(trifluoromethyl)phenyl!-3(2H)-pyridazinone;

orbencarb S- 2-(chlorophenyl)methyl!diethylcarbamothioate;

oryzalin 4-(dipropylamino)-3,5-dinitrobenzenesulfonamide;

oxadiazon 3- 2,4-dichloro-5-(1-methylethoxy)phenyl!-5-(1,1-dimethylethyl)-1,3,4-oxadiazol-2(3H)-one;

oxyfluorfen 2-chloro-1-(3-ethoxy-4-nitrophenoxy)-4-(trifluoromethyl)benzene;

paraquat 1,1'-dimethyl-4,4'-dipyridinium ion;

pebulate S-propyl butylethylcarbamothioate;

pendimethalin N-(1-ethylpropyl)-3,4-dimethyl-2,6-dinitrobenzenamine;

perfluidone 1,1-trifluoro-N- 2-methyl-4-(phenylsulfonyl)phenyl!methanesulfonamide;

phenisopham 3- (1-methylethoxy)carbonyl!amino!phenyl ethylphenylcarbamate;

phenmedipham 3- (methoxycarbonyl)amino!phenyl (3-methylphenyl)carbamate;

picloram 4-amino-3,5,6-trichloro-2-pyridinecarboxylic acid;

piperophos S- 2-(2-methyl-1-piperidinyl)-2-oxoethyl!O,O-dipropyl phosphorodithioate;

pirifenop-butyl butyl 2- 4- (3,5-dichloro-2-pyridinyl)oxy!phenoxy!propanoate;

PPG-1013 methyl 5- 2-chloro-4-(trifluoromethyl)phenoxy!-2-nitroacetophenone oxime O-acetate;

pretilachlor 2-chloro-N-(2,6-diethylphenyl)-N-(2-propoxyethyl)acetamide;

primisulfuron-methyl methyl 2- 4,6-bis(difluoromethoxy)pyrimidin-2-yl!amino!carbonyl!amino!sulfonyl!benzoate;

procyazine 2- 4-chloro-6-(cyclopropylamino)-1,3,5-triazine-2-yl!amino!-2-methylpropanenitrile;

prodiamine 2,4-dinitro-N³,N³ -dipropyl-6-(trifluoromethyl)-1,3-benzenediamine;

profluralin N-(cyclopropylmethyl)-2,6-dinitro-N-propyl-4-(trifluoromethyl)benzenamine;

proglinazine-ethyl ethyl N- 4-chloro-6- (1-methylethyl)amino!-1,3,5-triazin-2-yl!glycinate;

prometon 6-methoxy-N,N'-bis(1-methylethyl)-1,3,5-triazine-2,4-diamine;

prometryn N,N'-bis(1-methylethyl)-6-(methylthio)-1,3,5-triazine-2,4-diamine;

propachlor 2-chloro-N-(1-methylethyl)-N-phenylacetamide;

propanil N-(3,4-dichlorophenyl)propanamide;

propaquizafop 2- (1-methylethylidene)amino!oxy!ethyl 2- 4- (6-chloro-2-quinoxalinyl)oxy!phenoxy!propanoate;

propazine 6-chloro-N,N'-bis(1-methylethyl)-1,3,5-triazine2,4-diamine;

propham 1-methylethyl phenylcarbamate;

propyzamide 3,5-dichloro-N-(1,1-dimethyl-2-propynyl)benzamide;

prosulfalin N- 4-(dipropylamino)-3,5-dinitrophenyl!sulfonyl!-S,S-dimethylsulfilimine;

prosulfocarb S-(phenyl)methyl dipropylcarbamothioate;

prynachlor 2-chloro-N-(1-methyl-2-propynyl)acetanilide;

pyrazolynate 4-(2,4-dichlorobenzoyl)-1,3-dimethylpyrazol-5-yl!toluene-4-sulfonate;

pyrazon 5-amino-4-chloro-2-phenyl-3(2H)-pyridazinone;

pyrazosulfuron-ethyl 1-(4,6-dimethoxypyrimidin-2-yl)-3- (1-methyl)-4-(ethoxycarbonyl)pyrazol-5-yl!sulfonyl!urea;

pyrazoxyfen 2- 4-(2,4-dichlorobenzoyl)-1,3-dimethyl-1H-pyrazol-5-yl!oxy!-1-phenylethanone;

pyributicarb O- 3-(1,1-dimethylethyl)phenyl!(6-methoxy-2-pyridinyl)methylcarbamothioate;

pyridate O-(6-chloro-3-phenyl-4-pyridazinyl)S-octyl carbonothioate;

quinclorac 3,7-dichloro-8-quinolinecarboxylic acid;

quinmerac 7-chloro-3-methyl-8-quinolinecarboxylic acid;

quizalofop-ethyl ethyl 2- 4- (6-chloro-2-quinoxalinyl)oxy!phenoxy!propanoate;

S 275 2- 4-chloro-2-fluoro-5-(2-propynyloxy)phenyl!-4,5,6,7-tetrahydro-2H-indazole;

S 482 2- 7-fluoro-3,4-dihydro-3-oxo-4-(2-propynyl)-2H-1,4-benzoxazin-6-yl!-4,5,6,7-tetrahydro-1H-isoindole-1,3(2H)-dione;

secbumeton N-ethyl-6-methoxy-N'-(1-methylpropyl)-1,3,5-triazine-2,4-diamine;

sethoxydim 2- 1-(ethoxyimino)butyl!-5- 2-(ethylthio)propyl!-3-hydroxy-2-cyclohexen-1-one;

siduron N-(2-methylcyclohexyl)-N'-phenylurea;

simazine 6-chloro-N,N'-diethyl-1,3,5-triazine-2,4-diamine;

simetryn N,N'-diethyl-6-(methylthio)-1,3,5-triazine-2,4-diamine;

SN 106279 methyl 2- 7- 2-chloro-4-(trifluoromethyl)phenoxy!-2-naphthalenyl!oxy!propanoate;

sulfometuron-methyl methyl 2- (4,6-dimethyl-2-pyrimidinyl)amino!carbonyl!amino!sulfonyl!benzoate;

TCA trichloroacetic acid;

tebutam2,2-dimethyl-N-(1-methylethyl)-N-(phenylmethyl)propanamide;

tebuthiuron N- 5-(1,1-dimethylethyl)-1,3,4-thiadiazol-2-yl!-N,N'-dimethylurea;

terbacil 5-chloro-3-(1,1-dimethylethyl)-6-methyl-2,4(1H,3H)-pyrimidinedione;

terbucarb 2,6-bis(1,1-dimethylethyl)-4-methylphenyl methylcarbamate,

terbuchlor N-(butoxymethyl)-2-chloro-N- 2-(1,1-dimethylethyl)-6-methylphenyl!acetamide;

terbumeton N-(1,1-dimethylethyl)-N'-ethyl-6-methoxy-1,3,5-triazine-2,4-diamine;

terbuthylazine 6-chloro-N-(1,1-dimethylethyl)-N'-ethyl-1,3,5-triazine-2,4-diamine;

terbutryn N-(1,1-dimethylethyl)-N'-ethyl-6-(methylthio)-1,3,5-triazine-2,4-diamine;

TFH 450 N,N-diethyl-3- (2-ethyl-6-methylphenyl)-sulfonyl!-1H-1,2,4-triazole-1-carboxamide;

thiazafluron N,N'-dimethyl-N- 5-(trifluoromethyl)-1,3,4-thiadiazol-2-yl!-urea;

thifensulfuron-methyl methyl 3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)amino!carbonyl!amino!sulfonyl!thiophenecarboxylate;

thiobencarb S- (4-chlorophenyl)-methyl!-diethylcarbamothioate;

tiocarbazil S-(phenylmethyl)-bis(1-methylpropyl)carbamothioate;

tralkoxydim 2- 1-(ethoxyimino)propyl!-5- 2,4,6-trimethylphenyl!-3-hydroxy-2-cyclohexen-1-one;

tri-allate S-(2,3,3-trichloro-2-propenyl)bis(1-methylethyl)carbamothioate;

triasulfuron 1-(4-methoxy-6-methyl-1,3,5-triazin-2-yl)-3- 2-(2-chloroethoxy)phenylsulfonyl!urea;

triazofenamide 1-(3-methylphenyl)-5-phenyl-1,2,4-triazole-2-carboxamide;

tribenuron-methyl methyl 2- N-(4-methoxy-6-methyl-1,3,5-triazin-2-yl)-N-methylamino!carbonyl!amino!sulfonyl!benzoate;

triclopyr (3,5,6-trichloro-2-pyridinyl)oxy!acetic acid;

tridiphane 2-(3,5-dichlorophenyl)-2-(2,2,2-trichloroethyl)oxirane;

trietazine 6-chloro-N,N,N'-triethyl-1,3,5-triazine-2,4-diamine;

trifluralin 2,6-dinitro-N,N-dipropyl-4-(trifluoromethyl)benzenamine;

trimeturon 1-(4-chlorophenyl)-2,3,3-trimethylpseudourea;

vernolate S-propyl dipropylcarbamothioate;

WL 110547 5-phenoxy-1- 3-(trifluoromethyl)phenyl!-1H-tetrazole.

The active substance content of the use forms of the active substances can vary within wide ranges, for example from 0.0001 to 100% by weight of active substance, preferably 0,001 to 99% by weight of active substance.

The agrochemical preparations (formulations) generally contain 0.1 to 99 percent by weight, in particular 0.1 to 95% by weight, of herbicidal active substance, and 1 to 99.9% by weight, preferably 5 to 99.9% by weight, of formulation auxiliaries which are inert under the storage and use conditions.

The preparations are applied in a customary manner which suits the use forms.

For example, the formulations, present in commercially available form, are diluted for use, if appropriate, in a conventional manner, for example using water in the case of wettable powders, emulsifiable concentrates, dispersions and water-dispersible granules. Preparations in the form of dusts and granules and also sprayable solutions are usually not further diluted with other inert substances before use.

The required application rate of the compounds of the formula (I) according to the invention varies with the external conditions such as, inter alia, temperature, humidity, and nature of the herbicide used. It can be varied within wide limits, for example between 0.001 and 10.0 kg/ha or more of active ingredient, but it is preferably between 0.005 and 5 kg/ha.

A. CHEMICAL EXAMPLES Example 1 N-tert.-butyl-(2-iodo-3-methoxycarbonyl)benzenesulfonamide

A solution of 24.1 g of tert.-butylamine in 30 ml of dichloromethane is added dropwise at room temperature to 59.3 g of 2-iodo-3-methoxycarbonylbenzenesulfochloride in 300 ml of dichloromethane. Stirring is continued for 3 hours at room temperature, the mixture is washed with 2N hydrochloric acid and dried over Na₂ SO₄, and the solvent is evaporated. The residue is digested in ether. This gives 30.0 g of N-tert.-butyl-(2-iodo-3-methoxycarbonyl)benzenesulfonamide in the form of colorless crystals of m.p. 148°-9° C.

Example 2 2-Iodo-3-methoxycarbonylbenzenesulfonamide

27.9 g of N-tert.-butyl-(2-iodo-3-methoxycarbonyl)benzene-sulfonamide are stirred with 100 ml of trifluoroacetic acid for 4 hours at room temperature, the mixture is heated for 2 hours at the boil, and the organic phase is then evaporated in vacuo. The residue is taken up in dichloromethane/water, and sodium carbonate is added until the reaction is neutral. The phases are separated, and the aqueous phase is extracted two more times using dichloromethane. The combined organic phases are dried over Na₂ SO₄, and the solvent is evaporated. After stirring of the residue with ether, 17.4 g of 2-iodo-3-methoxycarbonylbenzenesulfonamide of m.p. 155°-7° C. are obtained.

Example 3 Methyl 2-amino-4-iodobenzoate

A solution of 16.1 g of 2-acetylamino-4-iodobenzoic acid (m.p. 233°-5° C; synthesized in accordance with U.S. Pat. No. 4,762,838) in 325 ml of absolute methanol is saturated at 0° C. with dry hydrogen chloride gas. The mixture is heated to the boil for 15 hours, cooled to room temperature, resaturated using dry hydrogen chloride gas, and allowed to stand at room temperature for 24 hours. The solvent is evaporated in vacuo, the residue is taken up in dichloromethane, and the organic phase is washed with a saturated aqueous sodium hydrogen carbonate solution until free from acid. The organic phase is dried over Na₂ SO₄, and evaporated in vacuo. This gives 13.8 g of methyl 2-amino-4-iodobenzoate of m.p. 63°-7° C.

Example 4 Bis(2-methoxycarbonyl-5-iodobenzene)disulfide

13.8 g of methyl 2-amino-4-iodobenzoate are treated with 48 ml of glacial acetic acid and subsequently with 86 ml of concentrated hydrochloric acid. A solution of 3.8 g of sodium nitrite in 15 ml of water is slowly added dropwise to this suspension which is cooled to -5° C., and stirring is continued at this temperature for 30 minutes. This cooled diazonium salt solution is added dropwise at 0° C. to a solution of 20 ml of sulfur dioxide, 60 ml of glacial acetic acid, 10 ml of water and 3.1 g of copper(II) chloride dihydrate, and stirring is continued first for 1 hour at 0° C. and then overnight at room temperature. The reaction mixture is poured into 1 l of ice-water, and the product is filtered off with suction. This gives 12.7 g of bis(2-methoxycarbonyl-5-iodobenzene)disulfide of m.p. 133°-5° C.

Example 5 2-Methoxycarbonyl-5-iodobenzenesulfochloride

Chlorine gas is passed at 20°-25° C. into 12.2 g of bis(2-methoxycarbonyl-5-iodobenzene)disulfide in a solution of 30 ml of 1,2-dichloroethane and 15 ml of 2N hydrochloric acid until the exothermic reaction has ended. The solids are filtered off with suction, the aqueous phase is extracted using dichloromethane, the combined organic phases are dried over Na₂ SO₄, and,the solvent is evaporated in vacuo. This gives a total amount of 15.0 g of 2-methoxycarbonyl-5-iodobenzenesulfochloride, from the filtered and extracted product, of m.p. 119°-120° C. (decomposition).

Example 6 2-Methoxycarbonyl-5-iodobenzenesulfonamide

Ammonia gas is passed at room temperature into 15.0 g of 2-methoxycarbonyl-5-iodobenzenesulfochloride in 100 ml of tetrahydrofuran until ammonia is no longer taken up. The solution is evaporated in vacuo, the residue is stirred thoroughly with water, and the product is filtered off with suction. After drying of the filter residue at 70° C. in vacuo, 10.7 g of 2-methoxycarbonyl-5-iodobenzenesulfonamide are obtained as a white powder of m.p. 176°-7° C.

Example 7 3-Ethoxycarbonyl-2-iodobenzenesulfochloride

24.0 g of ethyl 3-amino-2-iodobenzoate are dissolved in 60 ml of glacial acetic acid and 120 ml of concentrated hydrochloric acid. A solution of 6.9 g of sodium nitrite in 30 ml of water is slowly added dropwise to this suspension which is cooled to -5° C., and stirring is continued at this temperature for 30 minutes. This cooled diazonium salt solution is added dropwise at 5°-10° C. to a solution of 70 ml of glacial acetic acid, 70 ml of concentrated hydrochloric acid and 3.0 g of copper(II) chloride dihydrate, which has been saturated with sulfur dioxide at approx. 10° C. The mixture is stirred for 3 hours at room temperature, and chlorine gas is then passed in until the exothermic reaction subsides. The reaction mixture is poured into 1 l of ice-water, and the product is filtered off with suction and dried in vacuo at 50° C. This gives 25.3 g of 3-ethoxycarbonyl-2-iodobenzenesulfo-chloride of m.p. 80°-3° C.

Example 8 3-Ethoxycarbonyl-2-iodobenzenesulfonamide

Analogously to Example 6, 25.3 g of 3-ethoxycarbonyl-2-iodobenzenesulfochloride and ammonia gave 20.4 g of 3-ethoxycarbonyl-2-iodobenzenesulfonamide of m.p. 138°-9° C.

Example 9 Methyl 2- (4,6-dimethoxy-2-pyrimidinyl)amino!carbonyl!amino!sulfonyl!-4-iodobenzoate

A solution of 1.7 g of 1,8-diazabicyclo 5.4.0!undec-7-ene in 10 ml of absolute acetonitrile is added dropwise at room temperature to a mixture of 3.4 g of 5-iodo-2-methoxycarbonylbenzenesulfonamide and 2.8 g of O-phenyl (4,6-dimethoxy-2-pyrimidinyl)carbamate in 50 ml of absolute acetonitrile. The mixture is stirred at this temperature for 3 hours, concentrated to approx. 1/3 and poured into 200 ml of ice-water. The aqueous phase is extracted using diethyl ether, the pH is brought to 1-2 using concentrated hydrochloric acid, and the product is filtered off with suction. After drying in vacuo at 60° C., 3.3 g of methyl 2- (4,6-dimethoxy-2-pyrimidinyl)amino!carbonyl!amino!sulfonyl!-4-iodobenzoate of m.p. 169°-71° C. are obtained.

Example 10 Ethyl 2-iodo-3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)amino!carbonyl!amino!sulfonyl!benzoate

14 mmol of trimethylaluminum (7 ml of a 2M solution in hexane) are added dropwise under a nitrogen protective atmosphere to a suspension of 3.6 g of 3-ethoxycarbonyl-2-iodobenzenesulfonamide in 100 ml of absolute dichloromethane. The mixture is stirred at room temperature for 30 minutes, and 2.2 g of O-methyl (4-methyl-6-methoxy-1,3,5-triazin-2-yl)carbamate in 25 ml of dichloromethane are then added, and the mixture is refluxed for 13 hours. The solution is cooled to room temperature, 25 ml of 2N hydrochloric acid are added dropwise with ice-cooling, and the hydrochloric acid phase is extracted twice using dichloromethane. The organic phase is concentrated in vacuo, and the residue is treated with acetone and 100 ml of 10% aqueous sodium acetate solution. The mixture is stirred for 3 hours and then filtered off with suction, followed by a washing step with diethyl ether, the aqueous phase is brought to pH 2-3 using concentrated hydrochloric acid and stirred for 15 minutes, and the product is filtered off with suction. After drying in vacuo at 50° C., 1.7 g of ethyl 2-iodo-3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)amino!carbonyl!amino!sulfonyl!benzoate of m.p. 177°-9° C. are obtained.

Example 11 2-Methoxycarbonyl-5-iodobenzenesulfonyl isocyanate

50 g of the sulfonamide obtained in Example 6 are suspended in 150 ml of 1,2-dichloroethane and the suspension is treated with 27.7 ml of thionyl chloride. The mixture is heated at the boil for 4 hours, cooled to 50°-55° C. and treated with 0.5 ml of pyridine, and phosgene is passed for 31/2 hours into the solution which has now been brought to the boil. The mixture is concentrated under reduced pressure with the exclusion of moisture. The crude sulfonyl isocyanate which remains (52.6 g) crystallises upon standing.

Example 12 2-Iodo-3-methoxycarbonylbenzenesulfonyl isocyanate

27.3 g of 2-iodo-3-methoxycarbonylbenzenesulfonamide and 9.0 ml of n-butyl isocyanate in 300 ml of absolute acetone are treated with 12 ml of DBU at room temperature and heated at the boil for 3 hours. The reaction solution is cooled to room temperature, concentrated to approximately 1/3 of its volume and poured into 1 l of water. The aqueous phase is acidified with concentrated hydrochloric acid to a pH of 1-2, and the precipitate obtained is filtered off with suction. 31.3 g of methyl 2-iodo- (n-butylamino)carbonyl!amino!sulfonyl!benzoate of melting point 163°-7° C. are obtained.

29.0 g of the resulting butylsulfonylurea are suspended in 400 ml of chlorobenzene and the suspension is brought to the boil. Phosgene is then passed in at boiling heat. The resulting butyl isocyanate is distilled off slowly in the course of 5 hours over a 20 cm Vigreux column in the form of a mixture with chlorobenzene. The mixture is concentrated in vacuo with the exclusion of moisture. This gives 28.4 g of 2-iodo-3-methoxycarbonylbenzenesulfonyl isocyanate in the form of an oil.

The sulfonamides of Tables 1a and 1b are obtained analogously to the processes of Examples 1 to 8.

The sulfonylureas of Tables 2-6 are obtained analogously to the processes of Examples 9 and 10. In the tables, the abbreviations refer to the general formula which precedes each table.

The sulfonyl isocyanates of Tables 1c and 1d are obtained analogously to the processes of Examples 11 and 12.

                  TABLE 1a                                                         ______________________________________                                          ##STR12##                                                                     IIa   Q         R           I       M.p.  °C.!                          ______________________________________                                         a     O         CH.sub.3    2-I     155-7                                      b     O         CH.sub.2 CH.sub.3                                                                          2-I     138-9                                      c     O         CH.sub.2 CH.sub.2 CH.sub.3                                                                 2-I     130-1                                      d     O         CH(CH.sub.3).sub.2                                                                         2-I     133                                        e     O         CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        2-I                                                f     O         CH.sub.2 CH(CH.sub.3).sub.2                                                                2-I                                                g     O         CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              2-I                                                h     O         C(CH.sub.3).sub.3                                                                          2-I                                                i     O         CH.sub.2 CHCH.sub.2                                                                        2-I                                                j     O         CH.sub.2 C CH                                                                              2-I                                                k     O         CH.sub.2 CH.sub.2 Cl                                                                       2-I                                                l     O         CH.sub.2 CH.sub.2 OCH.sub.3                                                                2-I                                                m     O         c-C.sub.6 H.sub.11                                                                         2-I                                                n     O         CH.sub.3    6-I     161-2                                      o     O         CH.sub.2 CH.sub.3                                                                          6-I                                                p     O         CH.sub.2 CH.sub.2 CH.sub.3                                                                 6-I                                                q     O         CH(CH.sub.3).sub.2                                                                         6-I                                                r     O         CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        6-I                                                s     O         CH.sub.2 CH(CH.sub.3).sub.2                                                                6-I                                                t     O         CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              6-I                                                u     O         C(CH.sub.3).sub.3                                                                          6-I                                                v     O         CH.sub.2 CHCH.sub.2                                                                        6-I                                                w     O         CH.sub.2 C CH                                                                              6-I                                                x     O         CH.sub.2 CH.sub.2 Cl                                                                       6-I                                                y     O         CH.sub.2 CH.sub.2 OCH.sub.3                                                                6-I                                                z     O         c-C.sub.6 H.sub.11                                                                         6-I                                                ______________________________________                                    

                  TABLE 1b                                                         ______________________________________                                          ##STR13##                                                                     IIb   Q         R           I       M.p.  °C.!                          ______________________________________                                         a     O         CH.sub.3    3-I     194-6                                      b     O         CH.sub.2 CH.sub.3                                                                          3-I                                                c     O         CH.sub.2 CH.sub.2 CH.sub.3                                                                 3-I                                                d     O         CH(CH.sub.3).sub.2                                                                         3-I                                                e     O         CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        3-I                                                f     O         CH.sub.2 CH(CH.sub.3).sub.2                                                                3-I                                                g     O         CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              3-I                                                h     O         C(CH.sub.3).sub.3                                                                          3-I                                                i     O         CH.sub.2 CHCH.sub.2                                                                        3-I                                                j     O         CH.sub.2 C CH                                                                              3-I                                                k     O         CH.sub.2 CH.sub.2 Cl                                                                       3-I                                                l     O         CH.sub.2 CH.sub.2 OCH.sub.3                                                                3-I                                                m     O         c-C.sub.6 H.sub.11                                                                         3-I                                                n     O         CH.sub.3    5-I     181-182                                    o     O         CH.sub.2 CH.sub.3                                                                          5-I     162                                        p     O         CH.sub.2 CH.sub.2 CH.sub.3                                                                 5-I                                                q     O         CH(CH.sub.3).sub.2                                                                         5-I     139                                        r     O         CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        5-I                                                s     O         CH.sub.2 CH(CH.sub.3).sub.2                                                                5-I                                                t     O         CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              5-I                                                u     O         C(CH.sub.3).sub.3                                                                          5-I                                                v     O         CH.sub.2 CHCH.sub.2                                                                        5-I                                                w     O         CH.sub.2 C CH                                                                              5-I                                                x     O         CH.sub.2 CH.sub.2 Cl                                                                       5-I                                                y     O         CH.sub.2 CH.sub.2 OCH.sub.3                                                                5-I                                                z     O         c-C.sub.6 H.sub.11                                                                         5-I                                                aa    O         CH.sub.3    6-I     213-5                                      ab    O         CH.sub.2 CH.sub.3                                                                          6-I                                                ac    O         CH.sub.2 CH.sub.2 CH.sub.3                                                                 6-I                                                ad    O         CH(CH.sub.3).sub.2                                                                         6-I                                                ae    O         CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        6-I                                                af    O         CH.sub.2 CH(CH.sub.3).sub.2                                                                6-I                                                ag    O         CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              6-I                                                ah    O         C(CH.sub.3).sub.3                                                                          6-I                                                ai    O         CH.sub.2 CHCH.sub.2                                                                        6-I                                                aj    O         CH.sub.2 C CH                                                                              6-I                                                ak    O         CH.sub.2 CH.sub.2 Cl                                                                       6-I                                                al    O         CH.sub.2 CH.sub.2 OCH.sub.3                                                                6-I                                                am    O         c-C.sub.6 H.sub.11                                                                         6-I                                                ______________________________________                                    

                  TABLE 1c                                                         ______________________________________                                          ##STR14##                                                                     (VIa)  Q       R           I      IR band  cm.sup.-1 !                         ______________________________________                                         a      O       CH.sub.3    3-I    2225                                         b      O       CH.sub.2 CH.sub.3                                                                          3-I    2230                                         c      O       CH.sub.2 CH.sub.2 CH.sub.3                                                                 3-I    2225                                         d      O       CH(CH.sub.3).sub.2                                                                         3-I    2225                                         e      O       CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        3-I                                                 f      O       CH.sub.2 CH(CH.sub.3).sub.2                                                                3-I                                                 g      O       CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              3-I                                                 h      O       C(CH.sub.3).sub.3                                                                          3-I                                                 i      O       CH.sub.2 CHCH.sub.2                                                                        3-I                                                 j      O       CH.sub.2 C CH                                                                              3-I                                                 k      O       CH.sub.2 CH.sub.2 Cl                                                                       3-I                                                 l      O       CH.sub.2 CH.sub.2 OCH.sub.3                                                                3-I                                                 m      O       c-C.sub.6 H.sub.11                                                                         3-I                                                 n      O       CH.sub.3    5-I    2225                                         o      O       CH.sub.2 CH.sub.3                                                                          5-I                                                 p      O       CH.sub.2 CH.sub.2 CH.sub.3                                                                 5-I                                                 q      O       CH(CH.sub.3).sub.2                                                                         5-I                                                 r      O       CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        5-I                                                 s      O       CH.sub.2 CH(CH.sub.3).sub.2                                                                5-I                                                 t      O       CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              5-I                                                 u      O       C(CH.sub.3).sub.3                                                                          5-I                                                 v      O       CH.sub.2 CHCH.sub.2                                                                        5-I                                                 w      O       CH.sub.2 C CH                                                                              5-I                                                 x      O       CH.sub.2 CH.sub.2 Cl                                                                       5-I                                                 y      O       CH.sub.2 CH.sub.2 OCH.sub.3                                                                5-I                                                 z      O       c-C.sub.6 H.sub.11                                                                         5-I                                                 aa     O       CH.sub.3    6-I                                                 ab     O       CH.sub.2 CH.sub.3                                                                          6-I                                                 ac     O       CH.sub.2 CH.sub.2 CH.sub.3                                                                 6-I                                                 ad     O       CH(CH.sub.3).sub.2                                                                         6-I                                                 ae     O       CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        6-I                                                 af     O       CH.sub.2 CH(CH.sub.3).sub.2                                                                6-I                                                 ag     O       CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              6-I                                                 ah     O       C(CH.sub.3).sub.3                                                                          6-I                                                 ai     O       CH.sub.2 CHCH.sub.2                                                                        6-I                                                 aj     O       CH.sub.2 C CH                                                                              6-I                                                 ak     O       CH.sub.2 CH.sub.2 Cl                                                                       6-I                                                 al     O       CH.sub.2 CH.sub.2 OCH.sub.3                                                                6-I                                                 am     O       c-C.sub.6 H.sub.11                                                                         6-I                                                 ______________________________________                                    

                  TABLE 1d                                                         ______________________________________                                          ##STR15##                                                                     (VIb)  Q       R           I      IR band  cm.sup.-1 !                         ______________________________________                                         a      O       CH.sub.3    3-I    2230                                         b      O       CH.sub.2 CH.sub.3                                                                          3-I                                                 c      O       CH.sub.2 CH.sub.2 CH.sub.3                                                                 3-I                                                 d      O       CH(CH.sub.3).sub.2                                                                         3-I                                                 e      O       CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        3-I                                                 f      O       CH.sub.2 CH(CH.sub.3).sub.2                                                                3-I                                                 g      O       CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              3-I                                                 h      O       C(CH.sub.3).sub.3                                                                          3-I                                                 i      O       CH.sub.2 CHCH.sub.2                                                                        3-I                                                 j      O       CH.sub.2 C CH                                                                              3-I                                                 k      O       CH.sub.2 CH.sub.2 Cl                                                                       3-I                                                 l      O       CH.sub.2 CH.sub.2 OCH.sub.3                                                                3-I                                                 m      O       c-C.sub.6 H.sub.11                                                                         3-I                                                 n      O       CH.sub.3    5-I    2230                                         o      O       CH.sub.2 CH.sub.3                                                                          5-I    2225                                         p      O       CH.sub.2 CH.sub.2 CH.sub.3                                                                 5-I                                                 q      O       CH(CH.sub.3).sub.2                                                                         5-I    2225                                         r      O       CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        5-I                                                 s      O       CH.sub.2 CH(CH.sub.3).sub.2                                                                5-I                                                 t      O       CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              5-I                                                 u      O       C(CH.sub.3).sub.3                                                                          5-I                                                 v      O       CH.sub.2 CHCH.sub.2                                                                        5-I                                                 w      O       CH.sub.2 C CH                                                                              5-I                                                 x      O       CH.sub.2 CH.sub.2 Cl                                                                       5-I                                                 y      O       CH.sub.2 CH.sub.2 OCH.sub.3                                                                5-I                                                 z      O       c-C.sub.6 H.sub.11                                                                         5-I                                                 aa     O       CH.sub.3    6-I    222-5                                        ab     O       CH.sub.2 CH.sub.3                                                                          6-I                                                 ac     O       CH.sub.2 CH.sub.2 CH.sub.3                                                                 6-I                                                 ad     O       CH(CH.sub.3).sub.2                                                                         6-I                                                 ae     O       CH.sub.2 CH.sub.2 CH.sub.2 CH.sub.3                                                        6-I                                                 af     O       CH.sub.2 CH(CH.sub.3).sub.2                                                                6-I                                                 ag     O       CH(CH.sub.3)CH.sub.2 CH.sub.3                                                              6-I                                                 ah     O       C(CH.sub.3).sub.3                                                                          6-I                                                 ai     O       CH.sub.2 CHCH.sub.2                                                                        6-I                                                 aj     O       CH.sub.2 C CH                                                                              6-I                                                 ak     O       CH.sub.2 CH.sub.2 Cl                                                                       6-I                                                 al     O       CH.sub.2 CH.sub.2 OCH.sub.3                                                                6-I                                                 am     O       c-C.sub.6 H.sub.11                                                                         6-I                                                 ______________________________________                                    

                                      TABLE 2                                      __________________________________________________________________________      ##STR16##                                                                     Ex.                            M.p.                                            No.                                                                               Q R      R.sup.1                                                                           R.sup.2                                                                             R.sup.3                                                                             W Y Z  °C.!                                    __________________________________________________________________________     1  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 216-7                                           2  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 181-2                                           3  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N 133-4                                           4  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N 210                                             5  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N 201-2                                           6  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 7  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N 196 decomp.                                     8  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N 205-6                                           9  O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O CH                                                                               N 218-21                                          10 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 11 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N 192-3                                           12 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 13 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 14 O CH.sub.3                                                                              H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 15 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 16 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 17 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O N N                                                 18 O CH.sub.3                                                                              H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 19 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 20 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 21 O CH.sub.3                                                                              H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 22 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 23 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 24 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 25 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 26 O CH.sub.3                                                                              H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 27 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 28 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 29 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 30 O CH.sub.3                                                                              H  Cl   CH.sub.3                                                                            O N N                                                 31 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 32 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 33 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 34 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 35 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 36 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 37 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 38 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 39 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 40 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 41 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 42 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 43 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 44 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 45 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 46 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 47 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 48 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 49 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 50 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 51 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 52 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 53 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 54 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O N N                                                 55 O C.sub.2 H.sub.5                                                                       H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 56 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 57 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 58 O C.sub.2 H.sub.5                                                                       H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 59 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 60 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 61 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 62 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 63 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 64 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 65 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 66 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 67 O C.sub.2 H.sub.5                                                                       H  Cl   CH.sub.3                                                                            O N N                                                 68 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 69 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 70 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 71 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 72 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 73 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 74 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 75 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 76 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 77 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 78 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 79 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 80 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 81 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 82 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 83 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 84 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 85 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 86 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 87 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 88 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 89 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 90 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 91 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 92 O n-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 93 O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 94 O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 95 O n-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 96 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 97 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 98 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 99 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 100                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 101                                                                               O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 102                                                                               O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 103                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 104                                                                               O n-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 105                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 106                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 107                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 108                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 109                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 110                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 111                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 112                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 113                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 114                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 115                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 116                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 117                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 118                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 119                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 120                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 121                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 122                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 123                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 124                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 125                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 126                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 127                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 128                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 129                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 130                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 131                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 132                                                                               O i-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 133                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 134                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 135                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 136                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 137                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 138                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 139                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 140                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 141                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 142                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 143                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 144                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 145                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 146                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 147                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 148                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 149                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 150                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 151                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 152                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 153                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 154                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 155                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 156                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 157                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 158                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 159                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 160                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 161                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 162                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 163                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 164                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 165                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O N N                                                 166                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 167                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 168                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 169                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 170                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 171                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 172                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 173                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 174                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 175                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 176                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 177                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 178                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   CH.sub.3                                                                            O N N                                                 179                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 180                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 181                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 182                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 183                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 184                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 185                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 186                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 187                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 188                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 189                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 190                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 191                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 192                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 193                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 194                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 195                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 196                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 197                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 198                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 199                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 200                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 201                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 202                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O N N                                                 203                                                                               O CH.sub.2 C CH                                                                         H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 204                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 205                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 206                                                                               O CH.sub.2 C CH                                                                         H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 207                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 208                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 209                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 210                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 211                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 212                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 213                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 214                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 215                                                                               O CH.sub.2 C CH                                                                         H  Cl   CH.sub.3                                                                            O N N                                                 216                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 217                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 218                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 219                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 220                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 221                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 222                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 223                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 224                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 225                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 226                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 227                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 228                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 229                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 230                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 231                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 232                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 233                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 234                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 235                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 236                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 237                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 238                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 239                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 240                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 241                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 242                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 243                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 244                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 245                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 246                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 247                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 248                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 249                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 250                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 251                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 252                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 253                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 254                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 255                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 256                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 257                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 258                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 259                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 260                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 261                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 262                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 263                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 264                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 265                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 266                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 267                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 268                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 269                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 270                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 271                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 272                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 273                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 274                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 275                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 276                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 277                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 278                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 279                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N 211-3 decomp.                                   280                                                                               O CH.sub.3                                                                              H  CH.sub.3                                                                            SCH.sub.3                                                                           O N N 196-8                                           281                                                                               O CH.sub.3                                                                              H  c-C.sub.3 H.sub.5                                                                   OCH.sub.3                                                                           O N N 175-8                                           282                                                                               O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O N N 195-6                                           283                                                                               O CH.sub.3                                                                              H  CH.sub.2 SCH.sub.3                                                                  OCH.sub.3                                                                           O N N 147-50                                          284                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O N N 131-3                                           285                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N Na-salt                                                                        189                                             286                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N Na-salt                                                                        195                                             287                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N Na-salt                                                                        189                                             288                                                                               O CH.sub.3                                                                              H  c-C.sub.3 H.sub.5                                                                   CH.sub.3                                                                            O N N Na-salt                                                                        170                                             289                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O N N Na-salt                                                                        130                                             290                                                                               O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O N N Na-salt                                                                        172                                             291                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N Li-salt                                                                        124                                             292                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N Na-salt                                                                        191                                             293                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N Na-salt                                                                        118                                             294                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N Na-salt                                                                        138                                             295                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N Na-salt                                                                        184                                             __________________________________________________________________________

                                      TABLE 3                                      __________________________________________________________________________      ##STR17##                                                                     Ex.                                M.p.                                        No.                                                                               Q R      R.sup.1                                                                           R.sup.2 R.sup.3                                                                              W Y Z  °C.!                                __________________________________________________________________________     1  O CH.sub.3                                                                              H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N 169-71                                      2  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N 186-7                                       3  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N 172-3                                       4  O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N 195-6                                       5  O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N 177                                         6  O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             O N N 182-4                                       7  O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N 158-63                                      8  O CH.sub.3                                                                              H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N 174                                         9  O CH.sub.3                                                                              H  OCH.sub.3                                                                              Cl    O CH                                                                               N 170-2                                       10 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                            CH.sub.3                                                                             O CH                                                                               N                                             11 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                            OCF.sub.2 H                                                                          O CH                                                                               N 178-9                                       12 O CH.sub.3                                                                              H  OCH.sub.3                                                                              Br    O CH                                                                               N                                             13 O CH.sub.3                                                                              H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             14 O CH.sub.3                                                                              H  OCH.sub.3                                                                              SCH.sub.3                                                                            O CH                                                                               N                                             15 O CH.sub.3                                                                              H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O N N                                             16 O CH.sub.3                                                                              H  OCH.sub.3                                                                              OC.sub.3 H.sub.7                                                                     O CH                                                                               N                                             17 O CH.sub.3                                                                              H  OCH.sub.3                                                                              Cl    O N N                                             18 O CH.sub.3                                                                              H  Cl      OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             19 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                       OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             20 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                        OCH.sub.3                                                                            O CH                                                                               N                                             21 O CH.sub.3                                                                              H  CF.sub.3                                                                               OCH.sub.3                                                                            O CH                                                                               N                                             22 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                     CH.sub.3                                                                             O CH                                                                               N                                             23 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O CH                                                                               N                                             24 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.2 CF.sub.3                                                                   O CH                                                                               N                                             25 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N 125 decomp.                                 26 O CH.sub.3                                                                              H  OCH.sub.3                                                                              NHCH.sub.3                                                                           O N N                                             27 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N                                             28 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                        OC.sub.2 H.sub.5                                                                     O N N                                             29 O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             30 O CH.sub.3                                                                              H  Cl      CH.sub.3                                                                             O N N                                             31 O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             32 O CH.sub.3                                                                              H  OCH.sub.3                                                                              OCH.sub.3                                                                            S CH                                                                               N                                             33 O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             S CH                                                                               N                                             34 O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             S CH                                                                               N                                             35 O CH.sub.3                                                                              H  OCH.sub.3                                                                              OCH.sub.3                                                                            S N N                                             36 O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             S N N                                             37 O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             S N N                                             38 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N 174-7                                       39 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N 155-7                                       40 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N 163-4                                       41 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             42 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N 183-4                                       43 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             44 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N 168-70                                      45 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N 154-8                                       46 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              Cl    O CH                                                                               N 151-3                                       47 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                            CH.sub.3                                                                             O CH                                                                               N                                             48 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                            OCF.sub.2 H                                                                          O CH                                                                               N                                             49 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              Br    O CH                                                                               N                                             50 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             51 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              SCH.sub.3                                                                            O CH                                                                               N                                             52 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O N N                                             53 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OC.sub.3 H.sub.7                                                                     O CH                                                                               N                                             54 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              Cl    O N N                                             55 O C.sub.2 H.sub.5                                                                       H  Cl      OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             56 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                       OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             57 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                        OCH.sub.3                                                                            O CH                                                                               N                                             58 O C.sub.2 H.sub.5                                                                       H  CF.sub.3                                                                               OCH.sub.3                                                                            O CH                                                                               N                                             59 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                     CH.sub.3                                                                             O CH                                                                               N                                             60 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O CH                                                                               N                                             61 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.2 CF.sub.3                                                                   O CH                                                                               N                                             62 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N                                             63 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              NHCH.sub.3                                                                           O N N                                             64 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N                                             65 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                        OC.sub.2 H.sub.5                                                                     O N N                                             66 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             67 O C.sub.2 H.sub.5                                                                       H  Cl      CH.sub.3                                                                             O N N                                             68 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             69 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OCH.sub.3                                                                            S CH                                                                               N                                             70 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              CH.sub.3                                                                             S CH                                                                               N                                             71 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                               CH.sub.3                                                                             S CH                                                                               N                                             72 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OCH.sub.3                                                                            S N N                                             73 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              CH.sub.3                                                                             S N N                                             74 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                               CH.sub.3                                                                             S N N                                             75 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             76 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             77 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             78 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             79 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             80 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             81 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             82 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             83 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              Cl    O CH                                                                               N                                             84 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                            CH.sub.3                                                                             O CH                                                                               N                                             85 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                            OCF.sub.2 H                                                                          O CH                                                                               N                                             86 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              Br    O CH                                                                               N                                             87 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             88 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              SCH.sub.3                                                                            O CH                                                                               N                                             89 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O N N                                             90 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OC.sub.3 H.sub.7                                                                     O CH                                                                               N                                             91 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              Cl    O N N                                             92 O n-C.sub.3 H.sub.7                                                                     H  Cl      OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             93 O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                       OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             94 O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                        OCH.sub.3                                                                            O CH                                                                               N                                             95 O n-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                               OCH.sub.3                                                                            O CH                                                                               N                                             96 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     CH.sub.3                                                                             O CH                                                                               N                                             97 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O CH                                                                               N                                             98 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.2 CF.sub.3                                                                   O CH                                                                               N                                             99 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N                                             100                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              NHCH.sub.3                                                                           O N N                                             101                                                                               O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N                                             102                                                                               O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                        OC.sub.2 H.sub.5                                                                     O N N                                             103                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             104                                                                               O n-C.sub.3 H.sub.7                                                                     H  Cl      CH.sub.3                                                                             O N N                                             105                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             106                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            S CH                                                                               N                                             107                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             S CH                                                                               N                                             108                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             S CH                                                                               N                                             109                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            S N N                                             110                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             S N N                                             111                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             S N N                                             112                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N 190-1                                       113                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             114                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             115                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             116                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             117                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             118                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             119                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             120                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              Cl    O CH                                                                               N                                             121                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                            CH.sub.3                                                                             O CH                                                                               N                                             122                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                            OCF.sub.2 H                                                                          O CH                                                                               N                                             123                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              Br    O CH                                                                               N                                             124                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             125                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              SCH.sub.3                                                                            O CH                                                                               N                                             126                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O N N                                             127                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OC.sub.3 H.sub.7                                                                     O CH                                                                               N                                             128                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              Cl    O N N                                             129                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl      OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             130                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                       OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             131                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                        OCH.sub.3                                                                            O CH                                                                               N                                             132                                                                               O i-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                               OCH.sub.3                                                                            O CH                                                                               N                                             133                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     CH.sub.3                                                                             O CH                                                                               N                                             134                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O CH                                                                               N                                             135                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.2 CF.sub.3                                                                   O CH                                                                               N                                             136                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N                                             137                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              NHCH.sub.3                                                                           O N N                                             138                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N                                             139                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                        OC.sub.2 H.sub.5                                                                     O N N                                             140                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             141                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl      CH.sub.3                                                                             O N N                                             142                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             143                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            S CH                                                                               N                                             144                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             S CH                                                                               N                                             145                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             S CH                                                                               N                                             146                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            S N N                                             147                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             S N N                                             148                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             S N N                                             149                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             150                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             151                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             152                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             153                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             154                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             155                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             156                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             157                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              Cl    O CH                                                                               N                                             158                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                            CH.sub.3                                                                             O CH                                                                               N                                             159                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                            OCF.sub.2 H                                                                          O CH                                                                               N                                             160                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              Br    O CH                                                                               N                                             161                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             162                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              SCH.sub.3                                                                            O CH                                                                               N                                             163                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O N N                                             164                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OC.sub.3 H.sub.7                                                                     O CH                                                                               N                                             165                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              Cl    O N N                                             166                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl      OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             167                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                       OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             168                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                        OCH.sub.3                                                                            O CH                                                                               N                                             169                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CF.sub.3                                                                               OCH.sub.3                                                                            O CH                                                                               N                                             170                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                     CH.sub.3                                                                             O CH                                                                               N                                             171                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O CH                                                                               N                                             172                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.2 CF.sub.3                                                                   O CH                                                                               N                                             173                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N                                             174                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              NHCH.sub.3                                                                           O N N                                             175                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N                                             176                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                        OC.sub.2 H.sub.5                                                                     O N N                                             177                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             178                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl      CH.sub.3                                                                             O N N                                             179                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             180                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OCH.sub.3                                                                            S CH                                                                               N                                             181                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              CH.sub.3                                                                             S CH                                                                               N                                             182                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                               CH.sub.3                                                                             S CH                                                                               N                                             183                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              OCH.sub.3                                                                            S N N                                             184                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                              CH.sub.3                                                                             S N N                                             185                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                               CH.sub.3                                                                             S N N                                             186                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             187                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             188                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             189                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             190                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             191                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             192                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             193                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             194                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              Cl    O CH                                                                               N                                             195                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                            CH.sub.3                                                                             O CH                                                                               N                                             196                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                            OCF.sub.2 H                                                                          O CH                                                                               N                                             197                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              Br    O CH                                                                               N                                             198                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             199                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              SCH.sub.3                                                                            O CH                                                                               N                                             200                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OC.sub.2 H.sub.5                                                                     O N N                                             201                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OC.sub.3 H.sub.7                                                                     O CH                                                                               N                                             202                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              Cl    O N N                                             203                                                                               O CH.sub.2 C CH                                                                         H  Cl      OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             204                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                       OC.sub.2 H.sub.5                                                                     O CH                                                                               N                                             205                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                        OCH.sub.3                                                                            O CH                                                                               N                                             206                                                                               O CH.sub.2 C CH                                                                         H  CF.sub.3                                                                               OCH.sub.3                                                                            O CH                                                                               N                                             207                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                     CH.sub.3                                                                             O CH                                                                               N                                             208                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O CH                                                                               N                                             209                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.2 CF.sub.3                                                                   O CH                                                                               N                                             210                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N                                             211                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              NHCH.sub.3                                                                           O N N                                             212                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N                                             213                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                        OC.sub.2 H.sub.5                                                                     O N N                                             214                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             215                                                                               O CH.sub.2 C CH                                                                         H  Cl      CH.sub.3                                                                             O N N                                             216                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             217                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OCH.sub.3                                                                            S CH                                                                               N                                             218                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              CH.sub.3                                                                             S CH                                                                               N                                             219                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                               CH.sub.3                                                                             S CH                                                                               N                                             220                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              OCH.sub.3                                                                            S N N                                             221                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                              CH.sub.3                                                                             S N N                                             222                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                               CH.sub.3                                                                             S N N                                             223                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             224                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             225                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             226                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             227                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             228                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             229                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             230                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             231                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             232                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             233                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             234                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             235                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             236                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             237                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             238                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             239                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             240                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             241                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             242                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             243                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             244                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             245                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             246                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             247                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             248                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             249                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             250                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             251                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             252                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             253                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             254                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             255                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             256                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             257                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             258                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             259                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             260                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             261                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             262                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             263                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             264                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             265                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             266                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             267                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             268                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             269                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             270                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             271                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             272                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N                                             273                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             274                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N                                             275                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N                                             276                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                               CH.sub.3                                                                             O N N                                             277                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N                                             278                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N                                             279                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              SCH.sub.3                                                                            O N N 185-7                                       280                                                                               O CH.sub.3                                                                              H  SCH.sub.3                                                                              CH.sub.3                                                                             O N N 188                                         281                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              C.sub.2 H.sub.5                                                                      O N N 177-8                                       282                                                                               O CH.sub.3                                                                              H  c-C.sub.3 H.sub.5                                                                      OCH.sub.3                                                                            O N N 180-1                                       283                                                                               O CH.sub.3                                                                              H  CH.sub.2 SCH.sub.3                                                                     OCH.sub.3                                                                            O N N 108                                         284                                                                               O CH.sub.3                                                                              H  CH.sub.2 CH(OCH.sub.3).sub.2                                                           OCH.sub.3                                                                            O N N 137-8                                       285                                                                               O CH.sub.3                                                                              H                                                                                  ##STR18##                                                                             OCH.sub.3                                                                            O N N 157-8                                       286                                                                               O CH.sub.3                                                                              H  i-C.sub.3 H.sub.7                                                                      OCH.sub.3                                                                            O N N 164-5                                       287                                                                               O CH.sub.3                                                                              H  n-C.sub.3 H.sub.7                                                                      OCH.sub.3                                                                            O N N 154-5                                       288                                                                               O CH.sub.3                                                                              H  CH.sub.2 Cl                                                                            OCH.sub.3                                                                            O N N 178-9                                       289                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N 150-5                                       290                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH(OCH.sub.3).sub.2                                                                  O N N 108                                         291                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              SCH.sub.3                                                                            O N N 153-5                                       292                                                                               O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O N N 158-60                                      293                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O N N Na-salt                                                                        230-3                                       294                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N Na-salt                                                                        251-3                                       295                                                                               O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             O CH                                                                               N Na-salt                                                                        108                                         296                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N Na-salt                                                                        135                                         297                                                                               O CH.sub.3                                                                              H  CH.sub.3                                                                               CH.sub.3                                                                             O N N Na-salt                                                                        165                                         298                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N Na-salt                                                                        155                                         299                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N Li-salt                                                                        153                                         300                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH.sub.3                                                                             O N N K-salt                                                                         140                                         301                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N Na-salt                                                                        155                                         302                                                                               O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N Na-salt                                                                        150                                         303                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N Na-salt                                                                        160                                         304                                                                               O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                     OCH.sub.3                                                                            O N N Na-salt                                                                        110                                         305                                                                               O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                       NHCH.sub.3                                                                           O N N Na-salt                                                                        115                                         306                                                                               O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O CH                                                                               N Na-salt                                                                        115                                         307                                                                               O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              CH.sub.3                                                                             O CH                                                                               N Na-salt                                                                        145                                         308                                                                               O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              Cl    O CH                                                                               N Na-salt                                                                        150                                         309                                                                               O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                              CH.sub.3                                                                             O N N Na-salt                                                                        113                                         310                                                                               O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                              OCH.sub.3                                                                            O N N Na-salt                                                                        140                                         311                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              C.sub.2 H.sub.5                                                                      O N N Na-salt                                                                        132                                         312                                                                               O CH.sub.3                                                                              H  CH.sub.2 CH(OCH.sub.3).sub.2                                                           OCH.sub.3                                                                            O N N Na-salt                                                                        155                                         313                                                                               O CH.sub.3                                                                              H  CH.sub.2 SCH.sub.3                                                                     OCH.sub.3                                                                            O N N Na-salt                                                                        145                                         314                                                                               O CH.sub.3                                                                              H  i-C.sub.3 H.sub.7                                                                      OCH.sub.3                                                                            O N N Na-salt                                                                        155                                         315                                                                               O CH.sub.3                                                                              H  n-C.sub.3 H.sub.7                                                                      OCH.sub.3                                                                            O N N Na-salt                                                                        157                                         316                                                                               O CH.sub.3                                                                              H  CH.sub.2 Cl                                                                            OCH.sub.3                                                                            O N N Na-salt                                                                        185                                         317                                                                               O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O N N Na-salt                                                                        227-30                                      318                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                              CH(OCH.sub.3).sub.2                                                                  O N N Na-salt                                                                        135                                         319                                                                               O CH.sub.3                                                                              H  SCH.sub.3                                                                              CH.sub.3                                                                             O N N Na-salt                                                                        165                                         320                                                                               O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                              OCH.sub.3                                                                            O N N Na-salt                                                                        115                                         __________________________________________________________________________

                                      TABLE 4                                      __________________________________________________________________________      ##STR19##                                                                     Ex.                            M.p.                                            No.                                                                               Q R      R.sup.1                                                                           R.sup.2                                                                             R.sup.3                                                                             W Y Z  °C.!                                    __________________________________________________________________________     1  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 190-2                                           2  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 3  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 4  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 5  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 6  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 7  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 8  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 9  O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 10 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 11 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 12 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 13 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 14 O CH.sub.3                                                                              H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 15 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 16 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 17 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O N N                                                 18 O CH.sub.3                                                                              H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 19 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 20 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 21 O CH.sub.3                                                                              H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 22 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 23 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 24 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 25 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 26 O CH.sub.3                                                                              H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 27 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 28 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 29 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 30 O CH.sub.3                                                                              H  Cl   CH.sub.3                                                                            O N N                                                 31 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 32 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 33 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 34 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 35 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 36 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 37 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 38 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 39 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 40 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 41 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 42 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 43 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 44 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 45 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 46 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 47 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 48 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 49 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 50 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 51 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 52 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 53 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 54 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O N N                                                 55 O C.sub.2 H.sub.5                                                                       H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 56 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 57 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 58 O C.sub.2 H.sub.5                                                                       H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 59 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 60 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 61 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 62 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 63 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 64 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 65 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 66 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 67 O C.sub.2 H.sub.5                                                                       H  Cl   CH.sub.3                                                                            O N N                                                 68 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 69 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 70 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 71 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 72 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 73 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 74 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 75 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 76 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 77 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 78 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 79 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 80 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 81 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 82 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 83 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 84 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 85 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 86 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 87 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 88 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 89 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 90 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 91 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 92 O n-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 93 O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 94 O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 95 O n-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 96 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 97 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 98 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 99 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 100                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 101                                                                               O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 102                                                                               O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 103                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 104                                                                               O n-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 105                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 106                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 107                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 108                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 109                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 110                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 111                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 112                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 113                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 114                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 115                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 116                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 117                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 118                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 119                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 120                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 121                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 122                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 123                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 124                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 125                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 126                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 127                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 128                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 129                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 130                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 131                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 132                                                                               O i-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 133                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 134                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 135                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 136                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 137                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 138                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 139                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 140                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 141                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 142                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 143                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 144                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 145                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 146                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 147                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 148                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 149                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 150                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 151                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 152                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 153                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 154                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 155                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 156                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 157                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 158                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 159                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 160                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 161                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 162                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 163                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 164                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 165                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O N N                                                 166                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 167                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 168                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 169                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 170                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 171                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 172                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 173                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 174                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 175                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 176                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 177                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 178                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   CH.sub.3                                                                            O N N                                                 179                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 180                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 181                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 182                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 183                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 184                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 185                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 186                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 187                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 188                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 189                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 190                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 191                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 192                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 193                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 194                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 195                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 196                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 197                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 198                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 199                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 200                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 201                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 202                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O N N                                                 203                                                                               O CH.sub.2 C CH                                                                         H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 204                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 205                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 206                                                                               O CH.sub.2 C CH                                                                         H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 207                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 208                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 209                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 210                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 211                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 212                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 213                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 214                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 215                                                                               O CH.sub.2 C CH                                                                         H  Cl   CH.sub.3                                                                            O N N                                                 216                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 217                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 218                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 219                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 220                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 221                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 222                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 223                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 224                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 225                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 226                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 227                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 228                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 229                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 230                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 231                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 232                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 233                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 234                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 235                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 236                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 237                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 238                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 239                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 240                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 241                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 242                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 243                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 244                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 245                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 246                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 247                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 248                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 249                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 250                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 251                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 252                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 253                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 254                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 255                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 256                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 257                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 258                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 259                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 260                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 261                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 262                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 263                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 264                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 265                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 266                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 267                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 268                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 269                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 270                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 271                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 272                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 273                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 274                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 275                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 276                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 277                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 278                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 __________________________________________________________________________

                                      TABLE 5                                      __________________________________________________________________________      ##STR20##                                                                     Ex.                            M.p.                                            No.                                                                               Q R      R.sup.1                                                                           R.sup.2                                                                             R.sup.3                                                                             W Y Z  °C.!                                    __________________________________________________________________________     1  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 199-202                                         2  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 3  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 4  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N 212-5                                           5  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N 193-4                                           6  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N 196-7                                           7  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N 192                                             8  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 9  O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 10 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 11 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 12 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 13 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 14 O CH.sub.3                                                                              H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 15 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 16 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 17 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O N N                                                 18 O CH.sub.3                                                                              H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 19 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 20 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 21 O CH.sub.3                                                                              H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 22 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 23 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 24 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 25 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 26 O CH.sub.3                                                                              H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 27 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 28 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 29 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 30 O CH.sub.3                                                                              H  Cl   CH.sub.3                                                                            O N N                                                 31 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 32 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 33 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 34 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 35 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 36 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 37 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 38 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 182                                             39 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 40 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 41 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 42 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 43 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 44 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N 177-179                                         45 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 46 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 47 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 48 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 49 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 50 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 51 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 52 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 53 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 54 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O N N                                                 55 O C.sub.2 H.sub.5                                                                       H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 56 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 57 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 58 O C.sub.2 H.sub.5                                                                       H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 59 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 60 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 61 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 62 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 63 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 64 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 65 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 66 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 67 O C.sub.2 H.sub.5                                                                       H  Cl   CH.sub.3                                                                            O N N                                                 68 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 69 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 70 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 71 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 72 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 73 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 74 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 75 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 186-188                                         76 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 77 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 78 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 79 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 80 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 81 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N 107-108                                         82 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 83 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 84 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 85 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 86 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 87 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 88 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 89 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 90 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 91 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 92 O n-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 93 O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 94 O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 95 O n-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 96 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 97 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 98 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 99 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 100                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 101                                                                               O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 102                                                                               O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 103                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 104                                                                               O n-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 105                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 106                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 107                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 108                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 109                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 110                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 111                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 112                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 185                                             113                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 114                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 115                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 116                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 117                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 118                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N 150                                             119                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 120                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 121                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 122                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 123                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 124                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 125                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 126                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 127                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 128                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 129                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 130                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 131                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 132                                                                               O i-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 133                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 134                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 135                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 136                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 137                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 138                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 139                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 140                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 141                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 142                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 143                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 144                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 145                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 146                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 147                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 148                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 149                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 150                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 151                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 152                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 153                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 154                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 155                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 156                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 157                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 158                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 159                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 160                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 161                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 162                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 163                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 164                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 165                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O N N                                                 166                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 167                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 168                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 169                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 170                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 171                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 172                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 173                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 174                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 175                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 176                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 177                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 178                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   CH.sub.3                                                                            O N N                                                 179                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 180                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 181                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 182                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 183                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 184                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 185                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 186                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 187                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 188                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 189                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 190                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 191                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 192                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 193                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 194                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 195                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 196                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 197                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 198                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 199                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 200                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 201                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 202                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O N N                                                 203                                                                               O CH.sub.2 C CH                                                                         H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 204                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 205                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 206                                                                               O CH.sub.2 C CH                                                                         H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 207                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 208                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 209                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 210                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 211                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 212                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 213                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 214                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 215                                                                               O CH.sub.2 C CH                                                                         H  Cl   CH.sub.3                                                                            O N N                                                 216                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 217                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 218                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 219                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 220                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 221                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 222                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 223                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 224                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 225                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 226                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 227                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 228                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 229                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 230                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 231                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 232                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 233                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 234                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 235                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 236                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 237                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 238                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 239                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 240                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 241                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 242                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 243                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 244                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 245                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 246                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 247                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 248                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 249                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 250                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 251                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 252                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 253                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 254                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 255                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 256                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 257                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 258                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 259                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 260                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 261                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 262                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 263                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 264                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 265                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 266                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 267                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 268                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 269                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 270                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 271                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 272                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 273                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 274                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 275                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 276                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 277                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 278                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 279                                                                               O CH.sub.3                                                                              H  CH.sub.3                                                                            Cl   O CH                                                                               N 214-6 decomp.                                   280                                                                               O CH.sub.3                                                                              H  CH.sub.3                                                                            H    O CH                                                                               N 201-3 decomp.                                   281                                                                               O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N Na-salt                                                                        200                                             __________________________________________________________________________

                                      TABLE 6                                      __________________________________________________________________________      ##STR21##                                                                     Ex.                            M.p.                                            No.                                                                               Q R      R.sup.1                                                                           R.sup.2                                                                             R.sup.3                                                                             W Y Z  °C.!                                    __________________________________________________________________________     1  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N 173-177                                         2  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 3  O CH.sub.3                                                                              CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 4  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 5  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 6  O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 7  O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N 187-188                                         8  O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 9  O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 10 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 11 O CH.sub.3                                                                              H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 12 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 13 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 14 O CH.sub.3                                                                              H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 15 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 16 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 17 O CH.sub.3                                                                              H  OCH.sub.3                                                                           Cl   O N N                                                 18 O CH.sub.3                                                                              H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 19 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 20 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 21 O CH.sub.3                                                                              H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 22 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 23 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 24 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 25 O CH.sub.3                                                                              H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 26 O CH.sub.3                                                                              H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 27 O CH.sub.3                                                                              H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 28 O CH.sub.3                                                                              H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 29 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 30 O CH.sub.3                                                                              H  Cl   CH.sub.3                                                                            O N N                                                 31 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 32 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 33 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 34 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 35 O CH.sub.3                                                                              H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 36 O CH.sub.3                                                                              H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 37 O CH.sub.3                                                                              H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 38 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 39 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 40 O C.sub.2 H.sub.5                                                                       CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 41 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 42 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 43 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 44 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 45 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 46 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 47 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 48 O C.sub.2 H.sub.5                                                                       H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 49 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 50 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 51 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 52 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 53 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 54 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           Cl   O N N                                                 55 O C.sub.2 H.sub.5                                                                       H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 56 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 57 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 58 O C.sub.2 H.sub.5                                                                       H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 59 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 60 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 61 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 62 O C.sub.2 H.sub.5                                                                       H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 63 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 64 O C.sub.2 H.sub.5                                                                       H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 65 O C.sub.2 H.sub.5                                                                       H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 66 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 67 O C.sub.2 H.sub.5                                                                       H  Cl   CH.sub.3                                                                            O N N                                                 68 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 69 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 70 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 71 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 72 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 73 O C.sub.2 H.sub.5                                                                       H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 74 O C.sub.2 H.sub.5                                                                       H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 75 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 76 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 77 O n-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 78 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 79 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 80 O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 81 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 82 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 83 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 84 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 85 O n-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 86 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 87 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 88 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 89 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 90 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 91 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 92 O n-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 93 O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 94 O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 95 O n-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 96 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 97 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 98 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 99 O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 100                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 101                                                                               O n-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 102                                                                               O n-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 103                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 104                                                                               O n-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 105                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 106                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 107                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 108                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 109                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 110                                                                               O n-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 111                                                                               O n-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 112                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 113                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 114                                                                               O i-C.sub.3 H.sub.7                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 115                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 116                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 117                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 118                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 119                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 120                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 121                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 122                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 123                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 124                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 125                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 126                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 127                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 128                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           Cl   O N N                                                 129                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 130                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 131                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 132                                                                               O i-C.sub.3 H.sub.7                                                                     H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 133                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 134                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 135                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 136                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 137                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 138                                                                               O i-C.sub.3 H.sub.7                                                                     H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 139                                                                               O i-C.sub.3 H.sub.7                                                                     H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 140                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 141                                                                               O i-C.sub.3 H.sub.7                                                                     H  Cl   CH.sub.3                                                                            O N N                                                 142                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 143                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 144                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 145                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 146                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 147                                                                               O i-C.sub.3 H.sub.7                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 148                                                                               O i-C.sub.3 H.sub.7                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 149                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 150                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 151                                                                               O CH.sub.2 CHCH.sub.2                                                                   CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 152                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 153                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 154                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 155                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 156                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 157                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 158                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 159                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 160                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 161                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 162                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 163                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 164                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 165                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           Cl   O N N                                                 166                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 167                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 168                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 169                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 170                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 171                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 172                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 173                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 174                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 175                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 176                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 177                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 178                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  Cl   CH.sub.3                                                                            O N N                                                 179                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 180                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 181                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 182                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 183                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 184                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 185                                                                               O CH.sub.2 CHCH.sub.2                                                                   H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 186                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 187                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 188                                                                               O CH.sub.2 C CH                                                                         CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 189                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 190                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 191                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 192                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 193                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 194                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O CH                                                                               N                                                 195                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         CH.sub.3                                                                            O CH                                                                               N                                                 196                                                                               O CH.sub.2 C CH                                                                         H  OCF.sub.2 H                                                                         OCF.sub.2 H                                                                         O CH                                                                               N                                                 197                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Br   O CH                                                                               N                                                 198                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 199                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           SCH.sub.3                                                                           O CH                                                                               N                                                 200                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.2 H.sub.5                                                                    O N N                                                 201                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OC.sub.3 H.sub.7                                                                    O CH                                                                               N                                                 202                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           Cl   O N N                                                 203                                                                               O CH.sub.2 C CH                                                                         H  Cl   OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 204                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    OC.sub.2 H.sub.5                                                                    O CH                                                                               N                                                 205                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OCH.sub.3                                                                           O CH                                                                               N                                                 206                                                                               O CH.sub.2 C CH                                                                         H  CF.sub.3                                                                            OCH.sub.3                                                                           O CH                                                                               N                                                 207                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  CH.sub.3                                                                            O CH                                                                               N                                                 208                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O CH                                                                               N                                                 209                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.2 CF.sub.3                                                                  O CH                                                                               N                                                 210                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.2 CF.sub.3                                                                  OCH.sub.3                                                                           O N N                                                 211                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           NHCH.sub.3                                                                          O N N                                                 212                                                                               O CH.sub.2 C CH                                                                         H  OC.sub.2 H.sub.5                                                                    NHCH.sub.3                                                                          O N N                                                 213                                                                               O CH.sub.2 C CH                                                                         H  C.sub.2 H.sub.5                                                                     OC.sub.2 H.sub.5                                                                    O N N                                                 214                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 215                                                                               O CH.sub.2 C CH                                                                         H  Cl   CH.sub.3                                                                            O N N                                                 216                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 217                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S CH                                                                               N                                                 218                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S CH                                                                               N                                                 219                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S CH                                                                               N                                                 220                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           OCH.sub.3                                                                           S N N                                                 221                                                                               O CH.sub.2 C CH                                                                         H  OCH.sub.3                                                                           CH.sub.3                                                                            S N N                                                 222                                                                               O CH.sub.2 C CH                                                                         H  CH.sub.3                                                                            CH.sub.3                                                                            S N N                                                 223                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 224                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 225                                                                               O n-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 226                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 227                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 228                                                                               O n-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 229                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 230                                                                               O n-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 231                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 232                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 233                                                                               O i-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 234                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 235                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 236                                                                               O i-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 237                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 238                                                                               O i-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 239                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 240                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 241                                                                               O sec.-C.sub.4 H.sub.9                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 242                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 243                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 244                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 245                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 246                                                                               O sec.-C.sub.4 H.sub.9                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 247                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 248                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 249                                                                               O t-C.sub.4 H.sub.9                                                                     CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 250                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 251                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 252                                                                               O t-C.sub.4 H.sub.9                                                                     H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 253                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 254                                                                               O t-C.sub.4 H.sub.9                                                                     H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 255                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 256                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 257                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 258                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 259                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 260                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 261                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 262                                                                               O CH.sub.2 CH.sub.2 Cl                                                                  H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 263                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 264                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 265                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 266                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 267                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 268                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 269                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 270                                                                               O CH.sub.2 CH.sub.2 OCH.sub.3                                                           H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 271                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 272                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           OCH.sub.3                                                                           O CH                                                                               N                                                 273                                                                               O c-C.sub.6 H.sub.11                                                                    CH.sub.3                                                                          OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 274                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O CH                                                                               N                                                 275                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O CH                                                                               N                                                 276                                                                               O c-C.sub.6 H.sub.11                                                                    H  CH.sub.3                                                                            CH.sub.3                                                                            O N N                                                 277                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           CH.sub.3                                                                            O N N                                                 278                                                                               O c-C.sub.6 H.sub.11                                                                    H  OCH.sub.3                                                                           OCH.sub.3                                                                           O N N                                                 __________________________________________________________________________

B. FORMULATION EXAMPLES

a) A dust is obtained by mixing 10 parts by weight of a compound of the formula (I) and 90 parts by weight of talc as inert substance and comminuting the mixture in a hammer mill.

b) A wettable powder which is readily dispersible in water is obtained by mixing 25 parts by weight of a compound of the formula (I), 64 parts by weight of kaolin-containing quartz as inert substance, 10 parts by weight of potassium ligninsulfonate and 1 part by weight of sodium oleylmethyltauride as wetting and dispersing agent, and grinding the mixture in a pinned disk mill.

c) A dispersion concentrate which is readily dispersible in water is obtained by mixing 20 parts by weight of a compound of the formula (I) with 6 parts by weight of alkylphenol polyglycol ether ((R)Triton X 207), 3 parts by weight of isotridecanol polyglycol ether (8 EO) and 71 parts by weight of paraffinic mineral oil (boiling range for example approx. 255° up to above 277° C.), and grinding the mixture in a ball mill to a fineness of below 5 microns.

d) An emulsifiable concentrate is obtained from 15 parts by weight of a compound of the formula (I), 75 parts by weight of cyclohexane as solvent and 10 parts by weight of ethoxylated nonylphenol as emulsifier.

e) Water-dispersible granules are obtained by mixing

    ______________________________________                                         75 parts by weight of a compound of the formula (I),                           10 parts by weight of calcium ligninsulfonate,                                  5 parts by weight of sodium lauryl sulfate,                                    3 parts by weight of polyvinyl alcohol and                                     7 parts by weight of kaolin,                                                  ______________________________________                                    

grinding the mixture on a pinned disk mill, and granulating the powder in a fluidized bed by spraying on water as granulation liquid.

f) Alternatively, water-dispersible granules are obtained by homogenizing and precomminuting

    ______________________________________                                         25 parts by weight                                                                           of a compound of the formula (I),                                 5 parts by weight                                                                           of sodium 2,2'-dinaphthylmethane-                                              6,6'-disulfonate,                                                 2 parts by weight                                                                           of sodium oleylmethyltauride,                                     1 part by weight                                                                            of polyvinyl alcohol,                                            17 parts by weight                                                                           of calcium carbonate and                                         50 parts by weight                                                                           of water                                                         ______________________________________                                    

on a colloid mill, subsequently grinding the mixture on a bead mill, and atomizing and drying the resulting suspension in a spray tower by means of a single-substance nozzle.

g) Extruder granules are obtained by mixing 20 parts by weight of active substance, 3 parts by weight of sodium ligninsulfonate, 1 part by weight of carboxymethylcellulose and 76 parts by weight of kaolin, grinding the mixture and moistening it with water. This mixture is extruded and subsequently dried in a stream of air.

C. BIOLOGICAL EXAMPLES

The damage to the weed plants, or the tolerance by the crop plants, was scored using a key in which the effectiveness is expressed by figures from 0 to 5. The figures have the following meaning:

0=no effect or damage

1=0 to 20% effect or damage

2=20 to 40% effect or damage

3=40 to 60% effect or damage

4=60 to 80% effect or damage

5=80 to 100% effect or damage

1. Pre-emergence effect on weeds

Seeds or rhizome pieces of monocotyledon and dicotyledon weed plants were placed in sandy loam soil in plastic pots and covered with soil. The compounds according to the invention which were formulated in the form wettable powders or emulsion concentrates were then applied to the surface of the soil cover in the form of aqueous suspensions or emulsions at an application rate of 600-800 l of water/ha (converted), in various dosages. After the treatment, the pots were placed in a greenhouse and kept under good growth conditions for the weeds. After the test plants had emerged, the damage to the plants or the negative effect on the emergence was scored visually after a test period of 3 to 4 weeks by comparison with untreated controls. As shown by the score figures in Table 7, the compounds according to the invention have a good herbicidal pre-emergence action against a broad range of grass weeds and dicotyledon weeds.

                                      TABLE 7                                      __________________________________________________________________________     Pre-emergence effect                                                           Active substance                                                                       Dosage rate in                                                                        Herbicidal effect                                               Tab./Ex.                                                                               kg of ai/ha                                                                           STME                                                                               CRSE                                                                               SIAL                                                                              LOMU                                                                               ECCR                                                                               AVSA                                         __________________________________________________________________________     5/1     0.3    5   5   4  3   3   3                                            3/1     0.3    5   5   5  5   5   4                                            __________________________________________________________________________      Abbreviations:                                                                 STME = Stellaria media                                                         CRSE = Chrysanthemum segetum                                                   SIAL = Sinapis alba                                                            LOMU = Lolium multiflorum                                                      ECCR = Echinochloa crusgalli                                                   AVSA = Avena sativa                                                            a.i. = Active ingredient                                                 

Similarly good activities are generally also found in the case of the other compounds of Tables 2 to 7.

2. Post-emergence effect on weeds

Seeds or rhizome pieces of monocotyledon and dicotyledon weeds were placed in sandy loam soil in plastic pots, covered with soil and grown in a greenhouse under good growth conditions. Three weeks after sowing, the test plants were treated in the three-leaf stage.

The compounds according to the invention which were formulated as wettable powders or as emulsion concentrates were sprayed in various dosages on the green parts of the plants at an application rate of 600 to 800 l of water/ha (converted) and, after the test plants had remained in the greenhouse for about 3-4 weeks under ideal growth conditions, the effect of the preparations was scored visually by comparison with untreated controls.

The agents according to the invention also have a good herbicidal post-emergence action against a broad range of economically important grass weeds and dicotyledon weeds (Table 8).

                                      TABLE 8                                      __________________________________________________________________________     Post-emergence effect                                                          Active substance                                                                       Dosage rate in                                                                        Herbicidal effect                                               Tab./Ex.                                                                               kg of ai/ha                                                                           STME                                                                               CRSE                                                                               SIAL                                                                              LOMU                                                                               ECCR                                                                               AVSA                                         __________________________________________________________________________     3/1     0.3    5   5   5  5   5   2                                            __________________________________________________________________________      Abbreviations:                                                                 STME = Stellaria media                                                         CRSE = Chrysanthemum segetum                                                   SIAL = Sinapis alba                                                            LOMU = Lolium multiflorum                                                      ECCR = Echinochloa crusgalli                                                   AVSA = Avena sativa                                                            a.i. = Active ingredient                                                 

Similarly good activities are generally also found in the case of the other compounds of Tables 2 to 7. Compared with compounds of EP-A-7687 or U.S. Pat. No. 4,556,898, the compounds of the formula I according to the invention generally exhibit better activities against problem weeds such as Galium aparine or Echinochloa crus-galli.

3. Tolerance by crop plants

In further greenhouse experiments, seeds of a substantial number of crop plants and weeds were placed in sandy loam soil and covered with soil.

Some of the pots were treated immediately as described under 1., and the remaining pots were placed in a greenhouse until the plants had developed two to three true leaves and then sprayed with various dosages of the substances according to the invention, as described under 2.

Visual scoring four to five weeks after the application and after the plants had been in the greenhouse revealed that the compounds according on the invention did not inflict any damage on dicotyledon crops such as, for example, soya, cotton, oilseed rape, sugar beet and potatoes when used pre- and post-emergence, even when high dosages of active substance were used. Moreover, some substances also left Gramineae crops such as, for example, barley, wheat, rye, Sorghum species, maize or rice unharmed. The compounds according to the invention therefore have a high selectivity when used to control undesired plant growth in agricultural crops. Compared with the compound of U.S. Pat. No. 4,566,898 (cf. compound of the formula (3)) or Example 80 of EP-A-0,291,851, the compounds of the formula I according to the invention generally exhibit a better selectivity, in particular in the control of problem weeds such as Galium aparine or Echinochloa crus-galli in crops of useful plants.

4. Herbicidal effect when used in rice

Tubers and rhizomes or young plants or seeds of various rice weeds such as Cyperus species, Eleocharis, Scirpus and Echinochloa were placed or planted in sealed plastic pots containing special rice soil and flooded with water up to 1 cm above soil level. The same procedure was applied to rice plants.

Used pre-emergence, i.e. 3-4 days after transplanting, the compounds according to the invention were poured into the stagnant water in the form of aqueous suspensions or emulsions, or scattered into the water in the form of granules.

In each case three weeks later, the herbicidal effect and any harmful effect on rice were scored visually. The results show that the compounds according to the invention are suitable for selective weed control in rice.

Compared with rice herbicides existing to date, the compounds according to the invention are distinguished by the fact that they effectively control a large number of weeds which germinate from perennial organs, in particular also weeds which are difficult to control, while being tolerated by rice. 

We claim:
 1. A compound of the formula (I) and salts thereof, ##STR22## where Q is oxygen, sulfur or --N(R⁴)--,W is oxygen or sulfur, Y and Z independently of one another are CH or N, where Y and Z are not simultaneously CH, R is hydrogen; (C₁ -C₁₂)alkyl; (C₂ -C₁₀)alkenyl; (C₂ -C₁₀)alkynyl; (C₁ -C₆)alkyl, which is monosubstituted to tetrasubstituted by radicals selected from the group consisting of halogen, (C₁ -C₄)alkoxy-, (C₁ -C₄)thioalkyl, --CN, (C₂ -C₅)alkoxycarbonyl and (C₂ -C₆)alkenyl; (C₃ -C₈)cycloalkyl which is unsubstituted or substituted by radicals selected from the group consisting of (C₁ -C₄)alkyl, (C₁ -C₄)alkoxy, (C₁ -C₄)alkylthio and halogen; (C₅ -C₈)cycloalkenyl; phenyl(C₁ -C₄)alkyl which is unsubstituted or substituted in the phenyl radical; or a radical of the formulae A-1 to A-10 ##STR23## where X is O, S, S(O) or SO₂ ; R¹ is hydrogen or (C₁ -C₃)alkyl; R² is hydrogen, halogen, (C₁ -C₃)alkyl, (C₁ -C₃)alkoxy, where the two last-mentioned radicals are unsubstituted or monosubstituted or polysubstituted by halogen or (C₁ -C₃)alkoxy; R³ is hydrogen, halogen, (C₁ -C₃)alkyl, (C₁ -C₃)alkoxy or (C₁ -C₃)alkylthio, where the three last-mentioned radicals are unsubstituted or monosubstituted or polysubstituted by halogen or monosubstituted or disubstituted by (C₁ -C₃)alkoxy or (C₁ -C₃)alkylthio; or a radical of the formula NR⁵ R⁶, (C₃ -C₆)cycloalkyl, (C₂ -C₄)alkenyl, (C₂ -C₄)alkynyl, (C₃ -C₄)alkenyloxy or (C₃ -C₆)alkynyloxy; R⁴ is hydrogen, (C₁ -C₄)alkyl or (C₁ -C₄)alkoxy and R⁵ and R⁶ independently of one another are hydrogen, (C₁ -C₄)alkyl, (C₃ -C₄)alkenyl, (C₁ -C₄)haloalkyl or (C₁ -C₄)alkoxy.
 2. A compound or salts thereof as claimed in claim 1, whereinQ is O or S, W is O, Y is CH or N and Z is N.
 3. A compound or salts thereof as claimed in claim 1, whereinR is hydrogen; (C₁ -C₆)alkyl; (C₂ -C₆)alkenyl; (C₂ -C₆)alkynyl; (C₁ -C₄)alkyl which is monosubstituted to tetrasubstituted by radicals selected from the group consisting of halogen, (C₁ -C₂)alkoxy-, (C₁ -C₂)thioalkyl, (C₂ -C₃)alkoxycarbonyl and (C₂ -C₄)alkenyl; (C₅ -C₆)cycloalkyl which is unsubstituted or substituted by radicals selected from the group consisting of (C₁ -C₄)alkyl, (C₁ -C₄)alkoxy, (C₁ -C₄)alkylthio and halogen; (C₅ -C₆)cycloalkenyl; benzyl which is unsubstituted or substituted in the phenyl radical by one to three radicals selected from the group consisting of halogen, (C₁ -C₂)alkyl, (C₁ -C₂)alkoxy, (C₁ -C₂)haloalkyl, (C₁ -C₂)thioalkyl and (C₂ -C₄)alkoxycarbonyl, or a radical of the abovementioned formulae A-1 to A-10, where X is O, S, S(O) or SO₂.
 4. A compound of the formula (I) or salts thereof as claimed in claim 1, whereinR¹ is hydrogen or CH₃ ; R² is hydrogen, halogen, (C₁ -C₂)alkyl, (C₁ -C₂)alkoxy, where the two last-mentioned radicals are unsubstituted or monosubstituted or polysubstituted by halogen or (C₁ -C₃)alkoxy; R³ is hydrogen, halogen, (C₁ -C₂)alkyl, (C₁ -C₂)alkoxy or (C₁ -C₂)alkylthio, where the abovementioned alkyl-containing radicals are unsubstituted or monosubstituted or polysubstituted by halogen or monosubstituted or disubstituted by (C₁ -C₂)alkoxy or (C₁ -C₂)alkylthio; or a radical of the formula NR⁵ R⁶ ; R⁴ is hydrogen or (C₁ -C₂)alkyl and R⁵ and R⁶ independently of one another are hydrogen or (C₁ -C₂)alkyl.
 5. A compound or salts thereof as claimed in claim 1, whereinW is oxygen, R¹ is hydrogen or CH₃, Y is CH or N, Z is N, R² is hydrogen, CH₃, CH₂ CH₃, OCH₃, OCH₂ CH₃, or OCHF₂, Cl and R³ is hydrogen, CH₃, CH₂ CH₃, OCH₃, OCH₂ CH₃, or OCHF₂.
 6. A compound of formula (I) or salts thereof as claimed in claim 1, whereinQ is an oxygen atom, W is an oxygen atom or a sulfur atom, Y is CH or N, Z is N, R is hydrogen, (C₁ -C₆)alkyl, (C₂ -C₆)alkenyl, (C₂ -C₆)alkynyl, (C₁ -C₆)alkyl which is monosubstituted by halogen or (C₁ -C₂)alkoxy, or is (C₅ -C₆)cycloalkyl, or is benzyl, R¹ is hydrogen or methyl, R² is methoxy, ethoxy, OCF₃ H, OCH₂ CF₃, methyl, ethyl, halogen or CF₃, R³ is methoxy, ethoxy, OCF₂ H, OCH₂ CF₃, methylthio, methyl, ethyl, halogen, CF₃ or methylamino.
 7. A compound of formula (I) or salts thereof as claimed in claim 6, whereinW is an oxygen atom, R is (C₁ -C₆)alkyl, R¹ is hydrogen or methyl, R² is methoxy, OCF₂ H or methyl, and R³ is methoxy, OCF₂ H, methyl or chloro.
 8. A compound of formula (I) or salts thereof as claimed in claim 7, which ismethyl 2- (4,6-dimethoxy-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, ethyl 2- (4,6-dimethoxy-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, methyl 2- (4,6-dimethyl-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, ethyl 2- (4,6-dimethyl-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, methyl 4-iodo-2- (4-methoxy-6-methyl-2-pyrimidinyl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, ethyl 4-iodo-2- (4-methoxy-6-methyl-2-pyrimidinyl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, methyl 2- (4,6-dimethoxy-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, ethyl 2- (4-6-dimethoxy-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, methyl 2- (4,6-dimethyl-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, ethyl 2- (4,6-dimethyl-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-4-iodobenzoate or sodium salt thereof, methyl 4-iodo-2- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, or ethyl 4-iodo-2- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof.
 9. A compound of formula (I) or salts thereof as claimed in claim 7, which ismethyl 3- (4,6-dimethoxy-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, ethyl 3- (4,6-dimethoxy-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, methyl 2-iodo-3- (4-methoxy-6-methyl-2-pyrimidinyl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, ethyl 2-iodo-3- (4-methoxy-6-methyl-2-pyrimidinyl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, methyl 3- (4,6-dimethyl-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, ethyl 3- (4,6-dimethyl-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, methyl 3- (4,6-dimethoxy-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, ethyl 3- (4,6-dimethoxy-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, methyl 2-iodo-3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, ethyl 2-iodo-3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!-benzoate or sodium salt thereof, methyl 3- (4,6-dimethyl-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof, or ethyl 3- (4,6-dimethyl-1,3,5-triazin-2-yl)amino!-carbonyl!-amino!-sulfonyl!-2-iodobenzoate or sodium salt thereof.
 10. A compound of formula (I) or salts thereof as claimed in claim 7, which ismethyl 2- (4,6-dimethoxy-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-6-iodobenzoate or sodium salt thereof, ethyl 2- (4,6-dimethoxy-2-pyrimidinyl)-amino!carbonyl!-amino!-sulfonyl!-6-iodobenzoate or sodium salt thereof, ethyl 6-iodo-3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof, or methyl 6-iodo-3- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!benzoate or sodium salt thereof.
 11. An herbicidal or plant growth-regulating composition containing an effective amount of a compound of the formula (I) or a salt thereof as claimed in claim 1 and customary formulation auxiliaries.
 12. A method for controlling weeds which comprises using as an herbicide an effective amount of a compound of the formula (I) or a salt thereof as claimed in claim
 1. 13. A method as claimed in claim 12, which comprises applying an effective amount of the compound of formula (I) or salt thereof as claimed in claim 1 to the plants, seeds of the plants or to the area where they are grown.
 14. A method for regulating the growth of culture plants which comprises using as a plant-growth regulator an effective amount of a compound of the formula (I) or a salt thereof as claimed in claim
 1. 15. A method as claimed in claim 14, which comprises applying an effective amount of the compound of formula (I) or salt thereof as claimed in claim 1 to the plants, seeds of the plants or to the area where they are grown.
 16. A compound of formula (I) or salt thereof as claimed in claim 1, which is methyl-4-iodo-2- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!-amino!-sulfonyl!benzoate.
 17. A compound of formula (I) or salt thereof as claimed in claim 1, which is the sodium salt of methyl 4-iodo-2- (4-methoxy-6-methyl-1,3,5-triazin-2-yl)-amino!-carbonyl!amino!-sulfonyl!-benzoate. 